Palladium and organocatalysis: An excellent recipe for asymmetric synthesis

The dual activation of simple substrates by the combination of organocatalysis and palladium catalysis has been successfully applied in a variety of different asymmetric transformations. Thus, the asymmetric α-allylation of carbonyl compounds, α-fluorination of acyl derivatives, decarboxylative prot...

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Detalles Bibliográficos
Autores: Fernández-Ibañez, M. Ángeles, Maciá, Beatriz, Alonso, Diego A., Pastor, Isidro M.
Tipo de recurso: artículo
Fecha de publicación:2013
País:España
Institución:Universidad Autónoma de Madrid
Repositorio:Biblos-e Archivo. Repositorio Institucional de la UAM
Idioma:inglés
OAI Identifier:oai:repositorio.uam.es:10486/667528
Acceso en línea:http://hdl.handle.net/10486/667528
https://dx.doi.org/10.3390/molecules180910108
Access Level:acceso abierto
Palabra clave:Allylation
Asymmetric synthesis
Decarboxylative protonation
Dual activation
Fluorination
Organocatalysis
Palladium
Tandem reaction
Química
Descripción
Sumario:The dual activation of simple substrates by the combination of organocatalysis and palladium catalysis has been successfully applied in a variety of different asymmetric transformations. Thus, the asymmetric α-allylation of carbonyl compounds, α-fluorination of acyl derivatives, decarboxylative protonation of β-dicarbonyl compounds, cyclization reactions of alkynyl carbonyl compounds and β-functionalization of aldehydes have been efficiently achieved employing this double-catalytic methodology