Kinetic study of the degradation of ethiofencarb in aqueous solutions

A kinetic study of the hydrolysis of ethiofencarb (α-ethylthio-o-tolyl methylcarbamate) in pure water and in aqueous solutions at pH 2, 6, 9 and 12 and at three different temperatures (4, 20 and 50(± 1)°C) has been carried out using a gas chromatographic nitrogen-phosphorus detection method. The val...

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Bibliographic Details
Authors: Sanz-Asensio, J., Plaza-Medina, M., Martinez-Soria, M.T. [0000-0003-4208-2801]
Format: article
Status:Published version
Publication Date:1997
Country:España
Institution:Universidad de La Rioja (UR)
Repository:RIUR. Repositorio Institucional de la Universidad de La Rioja
OAI Identifier:oai:portal.dialnet.es:doc/5bbc69ccb750603269e821a3
Online Access:https://investigacion.unirioja.es/documentos/5bbc69ccb750603269e821a3
Access Level:Open access
Keyword:Ethiofencarb
Half-life
Hydrolysis
Reaction kinetics
Thermal degradation
Description
Summary:A kinetic study of the hydrolysis of ethiofencarb (α-ethylthio-o-tolyl methylcarbamate) in pure water and in aqueous solutions at pH 2, 6, 9 and 12 and at three different temperatures (4, 20 and 50(± 1)°C) has been carried out using a gas chromatographic nitrogen-phosphorus detection method. The values of the first-order rate constants (k) for the degradation reaction were calculated. The values for k were found to be dependent on pH and temperature. No acid hydrolysis was observed in any case. Complete degradation of ethiofencarb was observed at pH 12 at all three temperatures; it was practically instantaneous at room temperature. Ethiofencarb was also completely degraded at pH 9 at 20 and 50°C, while in pure water (pH 6) degradation took place at 50°C but not at 2°C. Ethiofencarb was not degraded in pure water at lower temperatures and, due to the reversible nature of the reaction, at equilibrium about 80% of the pesticide remained undegraded at room temperature.