Improved stability and spectral quality in ex situ dissolution DNP using an improved transfer device

Dissolution dynamic nuclear polarization (DNP) has become one of the predominant implementations for DNP. However, the technical implementation of transferring the sample from the polarizer to the nuclear magnetic resonance (NMR) system remains challenging. There is a need for additional technical o...

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Detalles Bibliográficos
Autores: Katsikis, Sotirios, Marín Montesinos, Ildefonso, Pons Vallès, Miquel, Ludwig, Christian, Günther, Ulrich L.
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2015
País:España
Institución:Universidad de Barcelona
Repositorio:Dipòsit Digital de la UB
OAI Identifier:oai:diposit.ub.edu:2445/138570
Acceso en línea:https://hdl.handle.net/2445/138570
Access Level:acceso abierto
Palabra clave:Espectroscòpia de ressonància magnètica nuclear
Polarització (Física nuclear)
Nuclear magnetic resonance spectroscopy
Polarization (Nuclear physics)
Descripción
Sumario:Dissolution dynamic nuclear polarization (DNP) has become one of the predominant implementations for DNP. However, the technical implementation of transferring the sample from the polarizer to the nuclear magnetic resonance (NMR) system remains challenging. There is a need for additional technical optimizations in order to use dissolution DNP for biochemical and chemical applications. Here we show how a newly designed pressure dissolution kit considerably improves spectral quality and stability by enabling highly reliable and fast sample transfer to the NMR system.