A betaine adduct of N-heterocyclic carbene and carbodiimide, an efficient ligand to produce ultra-small ruthenium nanoparticles

The betaine adduct of N-heterocyclic carbene and carbodiimide (ICy·(p-tol)NCN) was found to be a very efficient ligand to prepare very small (1–1.3 nm) ruthenium nanoparticles (RuNPs). The coordination of the ligand on the metal surface takes place through the carbodiimide moiety. The resulting RuNP...

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Detalhes bibliográficos
Autores: Martínez Prieto, Luis Miguel, Urbaneja, C., Palma Ramírez, María del Pilar, Cámpora Pérez, Juan, Philippot, Karine, Chaudret, Bruno
Formato: artículo
Estado:Versión enviada para evaluación y publicación
Fecha de publicación:2015
País:España
Recursos:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/66567
Acesso em linha:http://hdl.handle.net/11441/66567
https://doi.org/10.1039/C5CC00211G
Access Level:acceso abierto
Descrição
Resumo:The betaine adduct of N-heterocyclic carbene and carbodiimide (ICy·(p-tol)NCN) was found to be a very efficient ligand to prepare very small (1–1.3 nm) ruthenium nanoparticles (RuNPs). The coordination of the ligand on the metal surface takes place through the carbodiimide moiety. The resulting RuNPs led to decarbonylation of THF and showed size selectivity for styrene hydrogenation.