Synthesis and characterization of perovskite FAPbBr(3-x) I (x) thin films for solar cells

[EN] FAPbI3, FAPbBr3, and FAPbBr3-xIx perovskite thin films were produced in a single step from a solution containing a mixture of FAI, PbI2, FABr, and PbBr2 (FA = formamidinium). FAPbBr3-xIx perovskite thin films were deposited onto ITO-coated glass substrates by spin coating. X-ray diffraction ana...

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Detalles Bibliográficos
Autores: Slimi, B., Ben Assaker, I., Kriaa, A., Chtourou, R., Mollar García, Miguel Alfonso|||0000-0003-4315-0407, Marí, B.|||0000-0003-0001-419X
Tipo de recurso: artículo
Fecha de publicación:2017
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/101893
Acceso en línea:https://riunet.upv.es/handle/10251/101893
Access Level:acceso abierto
Palabra clave:Organic-inorganic perovskites
Formamidinium lead iodide
Formamidinium lead bromide
X-ray diffraction
Optical absorption
Photoluminescence
FISICA APLICADA
Descripción
Sumario:[EN] FAPbI3, FAPbBr3, and FAPbBr3-xIx perovskite thin films were produced in a single step from a solution containing a mixture of FAI, PbI2, FABr, and PbBr2 (FA = formamidinium). FAPbBr3-xIx perovskite thin films were deposited onto ITO-coated glass substrates by spin coating. X-ray diffraction analyses confirmed that these thin-film perovskites crystallize in the cubic phase (Pm-3 m) for all composition range 0 B x B 3. Mixed lead perovskites showed a high absorbance in the UV¿Vis range. The optical band gap was estimated from spectral absorbance measurements. It was found that the onset of the absorption edge for FAPbBr3¿xIx thin films ranges between 1.47 and 2.20 eV for x = 0 and x = 3, respectively. Photoluminescence emission energies for mixed halide perovskites were also dependent on their composition and presented intermediate values from 810.4 nm for FAPbI3 to 547.3 nm for FAPbBr3.