Frequency-dependent stimulated and post-stimulated voltage control of magnetism in transition metal nitrides

Magneto-ionics, which deals with the change of magnetic properties through voltage-driven ion migration, is expected to be one of the emerging technologies to develop energy-efficient spintronics. While a precise modulation of magnetism is achieved when voltage is applied, much more uncontrolled is...

Full description

Bibliographic Details
Authors: Tan, Zhengwei|||0000-0003-4142-0637, de Rojas, Julius|||0000-0002-1206-4744, Martins, Sofia|||0000-0002-1801-1651, Lopeandia, Aitor|||0000-0003-0566-8299, Quintana, Alberto|||0000-0002-9813-735X, Cialone, Matteo|||0000-0002-3018-2787, Herrero-Martín, Javier|||0000-0003-1986-8128, Meersschaut, Johan|||0000-0003-2467-1784, Vantomme, André|||0000-0001-9158-6534, Costa-Krämer, José L.|||0000-0002-7664-2195, Sort, Jordi|||0000-0003-1213-3639, Menéndez, Enric|||0000-0003-3809-2863
Format: article
Publication Date:2023
Country:España
Institution:Universitat Autònoma de Barcelona
Repository:Dipòsit Digital de Documents de la UAB
Language:English
OAI Identifier:oai:ddd.uab.cat:270889
Online Access:https://ddd.uab.cat/record/270889
https://dx.doi.org/urn:doi:10.1039/d2mh01087a
Access Level:Open access
Description
Summary:Magneto-ionics, which deals with the change of magnetic properties through voltage-driven ion migration, is expected to be one of the emerging technologies to develop energy-efficient spintronics. While a precise modulation of magnetism is achieved when voltage is applied, much more uncontrolled is the spontaneous evolution of magneto-ionic systems upon removing the electric stimuli (i.e., post-stimulated behavior). Here, we demonstrate a voltage-controllable N ion accumulation effect at the outer surface of CoN films adjacent to a liquid electrolyte, which allows for the control of magneto-ionic properties both during and after voltage pulse actuation (i.e., stimulated and post-stimulated behavior, respectively). This effect, which takes place when the CoN film thickness is below 50 nm and the voltage pulse frequency is at least 100 Hz, is based on the trade-off between generation (voltage ON) and partial depletion (voltage OFF) of ferromagnetism in CoN by magneto-ionics. This novel effect may open opportunities for new neuromorphic computing functions, such as post-stimulated neural learning under deep sleep.