Ruthenium-doped ZnO nanostructures: growth, characterization, and applications in waveguides and light-emitting devices

ZnO based materials are gaining importance due to its potential applications. In many of these applications, the size, shape and dopability of the structures grown play a determinant role. In the present work, ZnO nano- and microstructures doped with Ru have been grown using the Vapour-Solid (VS) me...

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Detalles Bibliográficos
Autores: Rodríguez Peña, Micaela, Sotillo Buzarra, Belén, Urbieta Quiroga, Ana Irene, Fernández Sánchez, Paloma
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/108961
Acceso en línea:https://hdl.handle.net/20.500.14352/108961
Access Level:acceso abierto
Palabra clave:538.9
ZnO:Ru
Zinc oxide
Ruthenium
Defects
Optical properties
Electron microscopy
Ciencias
Física del estado sólido
2211 Física del Estado Sólido
Descripción
Sumario:ZnO based materials are gaining importance due to its potential applications. In many of these applications, the size, shape and dopability of the structures grown play a determinant role. In the present work, ZnO nano- and microstructures doped with Ru have been grown using the Vapour-Solid (VS) method. Among the different growth parameters, gas flux and initial dopant content seem to play the major role to determine both shape and size of the structures. The main morphologies obtained are self-arranged triangular grids and elongated structures. Based on microscopic observations a simplified growth model is proposed for the grids. An exhaustive characterization has been performed. X-Ray diffraction (XRD) investigations demonstrate good crystallinity and texturing related to preferential growth direction changes due to doping. Luminescence characterization through photo- and cathodoluminescence (PL and CL) techniques reveals typical ZnO near band edge and deep level emission bands at 3.2 and 2.3 eV, respectively. The potential use of elongated structures as waveguides and optical cavities, Fabry-Pèrot resonators, is explored.