Aromatic ionene topology and counterion-tuned gelation of acidic aqueous solutions

Unusual gelation of acidic solutions was achieved using polycations bearing quaternary ammonium moieties. These ionene polymers are based on a disubstituted phenylene dibenzamide core, which allows the construction of different topomers (i.e. ortho-1, meta-2 and para-3). The topology of the polymers...

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Detalles Bibliográficos
Autores: Bachl, Jürgen, Bertran Cànovas, Òscar|||0000-0002-3689-1429, Mayr, Judith, Alemán Llansó, Carlos|||0000-0003-4462-6075, Díaz Díaz, David
Tipo de recurso: artículo
Fecha de publicación:2017
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/105556
Acceso en línea:https://hdl.handle.net/2117/105556
https://dx.doi.org/10.1039/c7sm00234c
Access Level:acceso abierto
Palabra clave:Polymers
Colloids
Polymerization
Polímers
Col·loides
Polimerització
Àrees temàtiques de la UPC::Enginyeria química
Descripción
Sumario:Unusual gelation of acidic solutions was achieved using polycations bearing quaternary ammonium moieties. These ionene polymers are based on a disubstituted phenylene dibenzamide core, which allows the construction of different topomers (i.e. ortho-1, meta-2 and para-3). The topology of the polymers was found to play a key role on their aggregation behaviour both in pure water and in a variety of aqueous acidic solutions leading to the formation of stable acidic gels. Specifically, ortho-1 showed superior gelation ability than the analogues meta-2 and para-3 in numerous solutions of different pH and ionic strengths. Lower critical gelation concentrations, higher gel-to-sol transition temperatures and faster gelation were usually observed for ortho-1 regardless the solvent system. Detailed computational molecular dynamic simulations revealed a major role of the counterion (Cl-) and specific polymer¿polymer interactions. In particular, hydrogen bonds, N–H¿p interactions and intramolecular p–p stacking networks are distinctive in ortho-1. In addition, counterions located at internal hydration regions also affect to such polymer¿polymer interactions, acting as binders and, therefore, providing additional stability.