Supercritical concentration of ethyl laurate from coconut oil

Countercurrent extractions with supercritical carbon dioxide (SCCO2) were carried out to fractionate ethyl laurate (EL) from a fatty acid ethyl ester (FAEE) mixture obtained by ethanolysis of coconut oil. The effect of pressure (9–14 MPa), temperature (40–70 °C) and CO2 flow rate (30–70 g/min) on th...

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Detalles Bibliográficos
Autores: Villanueva-Bermejo, David, Martín Hernández, Diego, Hurtado-Ribeira, Raúl, Hernández, Elvis Judith, Fornari Reale, Tiziana, Martín García, Diana, Vázquez de Frutos, Luis
Tipo de recurso: artículo
Fecha de publicación:2025
País:España
Institución:Universidad Autónoma de Madrid
Repositorio:Biblos-e Archivo. Repositorio Institucional de la UAM
Idioma:inglés
OAI Identifier:oai:repositorio.uam.es:10486/750541
Acceso en línea:https://hdl.handle.net/10486/750541
https://dx.doi.org/10.1016/j.lwt.2025.117928
Access Level:acceso abierto
Palabra clave:Coconut oil
ethyl laurate
fatty acid ethyl esters
fractionation
supercritical fluid extraction
Química
Descripción
Sumario:Countercurrent extractions with supercritical carbon dioxide (SCCO2) were carried out to fractionate ethyl laurate (EL) from a fatty acid ethyl ester (FAEE) mixture obtained by ethanolysis of coconut oil. The effect of pressure (9–14 MPa), temperature (40–70 °C) and CO2 flow rate (30–70 g/min) on the purity of ethyl laurate (EL-P) and long-chain saturated fatty acid ethyl esters (LCSFA-P) were investigated and modeled by Response Surface Methodology. Pressure had a positive effect on both responses. Higher temperatures led to larger EL-P, but lower LCSFA-P in the extracts. SCCO2 flow rate was only significant for EL-P and there was an interaction effect with temperature (highest EL-P achieved at the highest temperature and flow rate). The optimum experimental condition to reach a high EL-P and low LCSFA-P was 13 MPa, 70 °C and 70 g/min. The experimental EL-P and LCSFA-P achieved at that condition was 59.6 % and 14.2 %, respectively. The use of SCCO2 in a countercurrent column demonstrated to be a suitable technique that allowed obtaining an extract with an EL-P 20 % higher (enrichment factor of 1.2) and a LCSFA-P 50 % lower than those of the coconut oil used as feed. In addition, an EL recovery of 83.9 % was achieved