Passivation of Bi2Te3 topological insulator by transferred CVD-graphene

The investigation, and ultimate application, of topological insulators, typically involve exposure to ambient conditions or their integration with metals, which lead to surface oxidation or material intermixing. X-ray photoelectron spectroscopy (XPS) measurements that demonstrate passivated and inte...

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Detalles Bibliográficos
Autores: Galceran, Regina|||0000-0002-2080-2575, Bonell, Frédéric|||0000-0001-7296-0404, Camosi, Lorenzo, Sauthier, Guillaume|||0000-0003-3566-3878, Gebeyehu, Zewdu M.|||0000-0001-6451-6100, Esplandiu Egido, Maria José|||0000-0003-2079-0639, Arrighi, Aloïs|||0000-0002-9774-852X, Fernández Aguirre, Iván|||0000-0002-0123-1703, Figueroa García, Adriana Isabel|||0000-0002-8498-9383, Sierra, Juan F.|||0000-0002-5438-0534, Valenzuela, Sergio O.|||0000-0002-4632-8891
Tipo de recurso: artículo
Fecha de publicación:2022
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:273653
Acceso en línea:https://ddd.uab.cat/record/273653
https://dx.doi.org/urn:doi:10.1002/admi.202201997
Access Level:acceso abierto
Palabra clave:Bi2Te3
Graphene-topological insulator interface
Intermixing
Passivation
XPS
Descripción
Sumario:The investigation, and ultimate application, of topological insulators, typically involve exposure to ambient conditions or their integration with metals, which lead to surface oxidation or material intermixing. X-ray photoelectron spectroscopy (XPS) measurements that demonstrate passivated and intermixing-free interfaces in the topological insulator BiTe by means of dry-transferred CVD graphene are reported. After air exposure, no traces of BiTe oxidation are found. Furthermore, it is demonstrated that graphene acts as a very efficient metal and chalcogen diffusion barrier in BiTe/graphene/permalloy (Py) heterostructures, which are relevant for spintronics. Such results are in stark contrast with the significant surface degradation observed in bare BiTe under ambient conditions and the deep Bi-Te bonding disruption that occurs in BiTe/Py heterostructures. These findings provide a new approach to control and engineer topological insulator interfaces for spintronic applications and a new platform to investigate the combined use of graphene and topological insulator Dirac states.