Pd(II)-Catalyzed C-H Acylation of (Hetero)arenes. Recent Advances

Di(hetero)aryl ketones are important motifs present in natural products, pharmaceuticals or agrochemicals. In recent years, Pd(II)-catalyzed acylation of (hetero)arenes in the presence of an oxidant has emerged as a catalytic alternative to classical acylation methods, reducing the production of tox...

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Detalles Bibliográficos
Autores: Santiago Alvarez, Carlos, Sotomayor Anduiza, María Nuria, Lete Expósito, María Esther
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universidad del País Vasco
Repositorio:Addi. Archivo Digital para la Docencia y la Investigación
OAI Identifier:oai:addi.ehu.eus:10810/45827
Acceso en línea:http://hdl.handle.net/10810/45827
Access Level:acceso abierto
Palabra clave:C-H activation
acylation
palladium
arenes
heteroarenes
Descripción
Sumario:Di(hetero)aryl ketones are important motifs present in natural products, pharmaceuticals or agrochemicals. In recent years, Pd(II)-catalyzed acylation of (hetero)arenes in the presence of an oxidant has emerged as a catalytic alternative to classical acylation methods, reducing the production of toxic metal waste. Different directing groups and acyl sources are being studied for this purpose, although further development is required to face mainly selectivity problems in order to be applied in the synthesis of more complex molecules. Selected recent developments and applications are covered in this review.