Thermal stability and diffusion in gadolinium silicate gate dielectric films

Gadolinium silicate films on Si(100) annealed in oxygen and vacuum at temperatures up to 800 °C were analyzed by Rutherford backscattering and narrow resonance nuclear profiling. Oxygen diffused into the film eliminating oxygen vacancies, but Si diffusion, previously observed in Al and Y oxides and...

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Detalles Bibliográficos
Autores: Landheer, Dolf, Wu, Xiaohua, Morais, Jonder, Baumvol, Israel Jacob Rabin, Pezzi, Rafael Peretti, Miotti, Leonardo, Lennard, W.N., Kim, Joon-Kon
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2001
País:Brasil
Institución:Universidade Federal do Rio Grande do Sul (UFRGS)
Repositorio:Repositório Institucional da UFRGS
Idioma:inglés
OAI Identifier:oai:www.lume.ufrgs.br:10183/141228
Acceso en línea:http://hdl.handle.net/10183/141228
Access Level:acceso abierto
Palabra clave:Recozimento
Interdifusao quimica
Filmes finos dieletricos
Microscopia eletrônica
Compostos de gadolínio
Retroespalhamento rutherford
Auto-difusao
Estabilidade térmica
Descripción
Sumario:Gadolinium silicate films on Si(100) annealed in oxygen and vacuum at temperatures up to 800 °C were analyzed by Rutherford backscattering and narrow resonance nuclear profiling. Oxygen diffused into the film eliminating oxygen vacancies, but Si diffusion, previously observed in Al and Y oxides and in La and Zr silicate films, was absent. Higher-temperature annealing in oxygen resulted in the formation of an interfacial layer observable in high-resolution electron micrographs. Gd0.23Si0.14O0.63 films crystallize at temperatures between 1000 and 1050 °C. These observations combined with recent electrical measurements show that gadolinium silicate films may be a good candidate for the replacement of SiO2 in deep submicron metal–oxide–semiconductor gates.