Third-order nonlinear optical response of colloidal gold nanoparticles prepared by sputtering deposition

The nonlinear optical responses of gold nanoparticles dispersed in castor oil produced by sputtering deposition were investigated, using the thermally managed Z-scan technique. Particles with spherical shape and 2.6 nm of average diameter were obtained and characterized by transmission electron micr...

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Bibliographic Details
Authors: Castro, Hermerson Pablo Silva, Santos, Heberton Wender Luiz dos, Alencar, Marcio André Rodrigues Cavalcanti de, Teixeira, Sergio Ribeiro, Dupont, Jairton, Hickmann, Jandir Miguel
Format: article
Status:Published version
Publication Date:2013
Country:Brasil
Institution:Universidade Federal do Rio Grande do Sul (UFRGS)
Repository:Repositório Institucional da UFRGS
Language:English
OAI Identifier:oai:www.lume.ufrgs.br:10183/96578
Online Access:http://hdl.handle.net/10183/96578
Access Level:Open access
Keyword:Nanofabricação
Nanopartículas
Otica nao-linear
Colóides
Indice de refracao
Deposição por sputtering
Ouro
Microscopia eletrônica de transmissão
Description
Summary:The nonlinear optical responses of gold nanoparticles dispersed in castor oil produced by sputtering deposition were investigated, using the thermally managed Z-scan technique. Particles with spherical shape and 2.6 nm of average diameter were obtained and characterized by transmission electron microscopy and small angle X-ray scattering. This colloid was highly stable, without the presence of chemical impurities, neither stabilizers. It was observed that this system presents a large refractive third-order nonlinear response and a negligible nonlinear absorption. Moreover, the evaluation of the all-optical switching figures of merit demonstrated that the colloidal nanoparticles prepared by sputtering deposition have a good potential for the development of ultrafast photonic devices.