Metallic islands in the Kondo insulator SmB6

The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or n...

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Detalles Bibliográficos
Autores: Souza, J. C., Rosa, P. F.S., Sichelschmidt, J., Carlone, M. [UNESP], Venegas, P. A. [UNESP], Malcolms, M. O., Menegasso, P. M., Urbano, R. R., Fisk, Z., Pagliuso, P. G.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2020
País:Brasil
Institución:Universidade Estadual Paulista (UNESP)
Repositorio:Repositório Institucional da UNESP
Idioma:inglés
OAI Identifier:oai:repositorio.unesp.br:11449/221752
Acceso en línea:http://dx.doi.org/10.1103/PhysRevResearch.2.043181
http://hdl.handle.net/11449/221752
Access Level:acceso abierto
Descripción
Sumario:The predicted interplay between Kondo physics and nontrivial topology in SmB6 has stimulated many experimental reports, some of which are in apparent contradiction. The origin of the dispute may lie in the fragility of the Kondo insulating phase in the presence of Sm vacancies (Kondo holes) and/or natural impurities, such as Gd3+. In this work, we locally investigate this fragility for Al flux grown Sm1-xGdxB6 single crystals (0≤x≤0.02) by combining electron spin resonance (ESR) and complementary bulk measurements. The Gd3+ ESR spectra in a highly dilute regime (x∼0.0004) display the features of an insulating cubic environment. Remarkably, a metallic ESR line shape is observed for more concentrated samples (x≥0.004), even though these systems are still in a reasonably dilute regime and show insulating dc electrical resistivity. Our data indicate that the Kondo insulating state is destroyed locally around impurities before a global percolation occurs. This result not only explains the discrepancy between dc and ac conductivity but also provides a scenario to explain the presence of quantum oscillations in magnetization in the absence of quantum oscillations in electrical resistivity.