Microwave-assisted Passerini reactions under solvent-free conditions

Various α-acyloxy carboxyamides were easily obtained combining three building blocks in one step: a carboxylic acid, an aldehyde and an isonitrile (Passerini reaction), using microwave irradiation under solvent-free conditions. The products were obtained in good yields (61-90%) and in short reaction...

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Detalles Bibliográficos
Autores: Barreto, Angélica de Fátima S, Vercillo, Otilie E, Andrade, Carlos Kleber Z
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2011
País:Brasil
Institución:Universidade de Brasília (UnB)
Repositorio:Repositório Institucional da UnB
Idioma:inglés
OAI Identifier:oai:repositorio.unb.br:10482/28083
Acceso en línea:http://repositorio.unb.br/handle/10482/28083
https://dx.doi.org/10.1590/S0103-50532011000300008
Access Level:acceso abierto
Palabra clave:Α-aciloxi Carboxamidas
Reação Passerini
Irradiação por microondas
Reações sem solvente
Descripción
Sumario:Various α-acyloxy carboxyamides were easily obtained combining three building blocks in one step: a carboxylic acid, an aldehyde and an isonitrile (Passerini reaction), using microwave irradiation under solvent-free conditions. The products were obtained in good yields (61-90%) and in short reaction times (< 5 min), using two different temperatures (60 and 120 ºC). At 120 ºC, the yields were higher and the reactions faster (< 1 min). Most of the obtained products are multifunctional allowing their application in consecutive Passerini reactions