Surface-Analytical Studies of Supported Vanadium Oxide Monolayer Catalysts

Supported vanadium oxide catalysts consisting of surface vanadia species on oxide supports were investigated by X-ray photoelectron spectroscopy  XPS and ion scattering spectroscopy ISS to elucidate the effect of calcintion temepratures as well as exposures to X-rays and He ions on the surface prope...

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Detalles Bibliográficos
Autores: Briand, Laura Estefania, Tkachenko, Olga Petrovna, Guraya, Monica, Gao, Xingtao, Wachs, Israel E., Grunert, Wolfgang
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2004
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/61927
Acceso en línea:http://hdl.handle.net/11336/61927
Access Level:acceso abierto
Palabra clave:Vanadium Monolayer
Surface Science
Ion Scattering Spectroscopy
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descripción
Sumario:Supported vanadium oxide catalysts consisting of surface vanadia species on oxide supports were investigated by X-ray photoelectron spectroscopy  XPS and ion scattering spectroscopy ISS to elucidate the effect of calcintion temepratures as well as exposures to X-rays and He ions on the surface properties. It was found that in supported V2O5/ZrO2, V2O5/CeO2 and V2O5/Nb2O5 catalysts possessing a vanadia monolayer coverage or above, the supports are densely covered by two-dimensional surface vanadia species, and the underlaying oxide support cations are not exposed. For a supported V2O5/Al2O3 catalyst containing  however, a slight exposure of the oxide support cation Al was noted, which may originate from the much higher surface area of the support and resulting in a higher curvature of the surfaces covered by supported vanadia species.