On-surface synthesis of metal-organic frameworks: the critical role of the reaction conditions

Two different metal-organic frameworks with either a honeycomb or Kagome structure were grown on Cu(111) using para-aminophenol molecules and native surface adatoms. Although both frameworks are made up from the same chemical species, they are structurally different emphasizing the critical role bei...

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Detalles Bibliográficos
Autores: Ruiz del Árbol, Nerea, Sánchez Sánchez, Carlos, Martínez, José I., Rodriguez, Luis Miguel, Serrate, David, Verdini, Alberto, Floreano, Luca, Jacobson, Peter, Grill, Leonhard, Martín Gago, José Ángel, López, María F.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2023
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/228526
Acceso en línea:http://hdl.handle.net/11336/228526
Access Level:acceso abierto
Palabra clave:metal-organic framewok
on-surface synthesis
STM
XPS
https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
Descripción
Sumario:Two different metal-organic frameworks with either a honeycomb or Kagome structure were grown on Cu(111) using para-aminophenol molecules and native surface adatoms. Although both frameworks are made up from the same chemical species, they are structurally different emphasizing the critical role being played by the reaction conditions during their growth. This work highlights the importance of the balance between thermodynamics and kinetics in the final structure of surface-supported metal-organic networks.