Non-competitive reversible inhibition of laccase by H2O2 in osmium mediated layer-by-layer multilayer O2 biocathodes

A systematic study of the inhibition of laccase by hydrogen peroxide in oxygen biocathodes composed of layer-by-layer selfassembled multilayers of Trametes-trogii laccase and osmium derivatized poly(allylamine) redox mediator has been accomplished using a rotating disc electrode at different electro...

Descripción completa

Detalles Bibliográficos
Autores: Grattieri, Matteo, Scodeller, Pablo David, Adam, Catherine, Calvo, Ernesto Julio
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2015
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/59233
Acceso en línea:http://hdl.handle.net/11336/59233
Access Level:acceso abierto
Palabra clave:Laccase
Oxygen
Peroxide
Inhibition
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descripción
Sumario:A systematic study of the inhibition of laccase by hydrogen peroxide in oxygen biocathodes composed of layer-by-layer selfassembled multilayers of Trametes-trogii laccase and osmium derivatized poly(allylamine) redox mediator has been accomplished using a rotating disc electrode at different electrode potentials, oxygen partial pressures and hydrogen peroxide concentrations. The experimental results are consistent with a reversible non-competitive inhibition mechanism in agreement with the Solomon mechanism for laccase previously reported.