Sizing gold nanoparticles by optical extinction spectroscopy

The measurement of optical extinction is used to determine the size of nearly spherical gold nanoparticles suspended in solution, produced by a 'reverse micelles' process. The contrast between the maximum and the minimum in the extinction spectra around 450 and 520 nm shows a linear depend...

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Detalles Bibliográficos
Autores: Scaffardi, Lucía Beatriz, Pellegrini, María Celeste, de Sanctis, O., Tocho, Jorge Omar
Tipo de recurso: artículo
Estado:Versión enviada para evaluación y publicación
Fecha de publicación:2005
País:Argentina
Institución:Comisión de Investigaciones Científicas de la Provincia de Buenos Aires
Repositorio:CIC Digital (CICBA)
Idioma:inglés
OAI Identifier:oai:digital.cic.gba.gob.ar:11746/559
Acceso en línea:https://digital.cic.gba.gob.ar/handle/11746/559
Access Level:acceso abierto
Palabra clave:Ciencias Físicas
accelerators
beams and electromagnetism
condensed matter
Nanoscale science and low-D systems
Descripción
Sumario:The measurement of optical extinction is used to determine the size of nearly spherical gold nanoparticles suspended in solution, produced by a 'reverse micelles' process. The contrast between the maximum and the minimum in the extinction spectra around 450 and 520 nm shows a linear dependence with the mean radius of the gold particles less than 3 nm; however, the method can be used to size particles up to 7 nm. Experimental results for extinction spectra can be fitted by Mie's theory if the optical constants from bulk material values are modified by introducing the limitation of the mean free path due to collisions of conduction electrons with the boundary of the nanoparticles.