Toughened Polystyrene Nanoparticles through High-Solids Miniemulsion Polymerization

Polystyrene nanoparticles toughened with polybutadiene were synthesized by miniemulsion polymerization of 50% solids content. The effects of recipes and reaction conditions on the polymerization kinetics, polymer microstructure, particle morphology, and mechanical properties of the produced thermopl...

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Bibliographic Details
Authors: Ronco, Ludmila Irene, Minari, Roque Javier, Passeggi, Mario Cesar Guillermo, Meira, Gregorio Raul, Gugliotta, Luis Marcelino
Format: article
Status:Published version
Publication Date:2015
Country:Argentina
Institution:Consejo Nacional de Investigaciones Científicas y Técnicas
Repository:CONICET Digital (CONICET)
Language:English
OAI Identifier:oai:ri.conicet.gov.ar:11336/4400
Online Access:http://hdl.handle.net/11336/4400
Access Level:Open access
Keyword:Miniemulsion Polymerization
High-Solids Content
Toughened Polystyrene
Polybutadiene
https://purl.org/becyt/ford/2.10
https://purl.org/becyt/ford/2
Description
Summary:Polystyrene nanoparticles toughened with polybutadiene were synthesized by miniemulsion polymerization of 50% solids content. The effects of recipes and reaction conditions on the polymerization kinetics, polymer microstructure, particle morphology, and mechanical properties of the produced thermoplastic materials, are discussed. The final material characteristics are strongly dependant on the chemical nature of the employed initiator, and an interpretation for the observed effects is presented. The obtained nanostructured polystyrenes exhibit mechanical properties similar to those of the commercial HIPS, but with the typical advantages of polymerizations in disperse medium such as low environmental impact, high monomer conversion, and fast heat transfer.