Particle Nucleation Using Different Initiators in the Miniemulsion Polymerization of Styrene

In miniemulsion polymerization, droplets nucleation is the key factor to ensure the production of polymer particles with a desired composition. The influence of the initiation on droplets nucleation is even conflicting and it has not been completely considered. The result of employing different init...

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Detalles Bibliográficos
Autores: Ronco, Ludmila Irene, Minari, Roque Javier, Gugliotta, Luis Marcelino
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2015
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/9012
Acceso en línea:http://hdl.handle.net/11336/9012
Access Level:acceso abierto
Palabra clave:Miniemulsion polymerization
Particle nucleation
polystyrene
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descripción
Sumario:In miniemulsion polymerization, droplets nucleation is the key factor to ensure the production of polymer particles with a desired composition. The influence of the initiation on droplets nucleation is even conflicting and it has not been completely considered. The result of employing different initiators systems on the nucleation mechanism and kinetics in the polymerization of stable styrene/polystyrene miniemulsions with varied droplets size is here discussed. The employed initiation systems provide all combinations between the phase (aqueous or organic) where initiation mainly occurs and the phase affinity of the produced radicals. Latexes with different contribution of the droplets nucleation were synthesized according to the employed initiation system and the droplets size of the miniemulsion. The results here presented could be used as a guide for choosing the initiation system to achieve the required contribution of the droplets nucleation.