Degradation of polycaprolactone/starch blends and composites with sisal fibre

The susceptibility of polycaprolactone/starch (PCL/S) and sisal fibre-reinforced polycaprolactone/starch blends (SF-PCL/S) to different degrading environments was evaluated. The composites and the unfilled matrix showed hydrolytic stability at pH 7.2 at two different temperatures (25 °C and 40 °C)....

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Detalles Bibliográficos
Autores: Di Franco, C.R., Cyras, Viviana Paola, Busalmen, Juan Pablo, Ruseckaite, Roxana Alejandra, Vázquez, A.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2004
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/94395
Acceso en línea:http://hdl.handle.net/11336/94395
Access Level:acceso abierto
Palabra clave:DEGRADATION
HYDROLYSIS
POLYCAPROLACTONE
SISAL FIBRE
SOIL BURIAL
STARCH
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descripción
Sumario:The susceptibility of polycaprolactone/starch (PCL/S) and sisal fibre-reinforced polycaprolactone/starch blends (SF-PCL/S) to different degrading environments was evaluated. The composites and the unfilled matrix showed hydrolytic stability at pH 7.2 at two different temperatures (25 °C and 40 °C). Fibres were stable under hydrolytic conditions and seemed to favour the entrance of water and then, the swelling and the hydrolysis of the starch (the most bio-available component). At higher fibre content, the composites become more hydrolytically stable probably due to the presence of a fibre–fibre physical network. Microbial attack in biotic aqueous medium was evidenced by the presence of a biofilm, especially on the fibre surface. In soil burial, PCL/S and 15%SF–PCL/S were degraded to about 50% of the initial mass. The weight loss pattern showed by the composite was associated with the presence of strong fibre–fibre and fibre–matrix interactions, which are absent in the neat matrix.