Theoretical Study of a New Diarylic Ligand for M2+ Cations Detection

A novel diarylic ligand developed as chemosensor for the detection of M2+ was studied by density functional theory (DFT) and time-dependent DFT (TD-DFT). Geometries of the free-ligand and M2+-ligand complex were optimized at the CAM-B3LYP/631+G(d,p) level of theory in dimethyl sulfoxide using the co...

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Detalles Bibliográficos
Autores: Ormachea, Carla, Ferretti, Cristián Alejandro, Noriega, Pablo, Marchi, Alberto Julio, Mancini, Pedro Maximo Emilio, Kneeteman, Maria Nelida
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2019
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/118566
Acceso en línea:http://hdl.handle.net/11336/118566
Access Level:acceso abierto
Palabra clave:CHEMOSENSOR
DFT
CU 2+ ION
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descripción
Sumario:A novel diarylic ligand developed as chemosensor for the detection of M2+ was studied by density functional theory (DFT) and time-dependent DFT (TD-DFT). Geometries of the free-ligand and M2+-ligand complex were optimized at the CAM-B3LYP/631+G(d,p) level of theory in dimethyl sulfoxide using the conductor like polarizable continuum model. The adsorption spectra of these molecules were analyzed and compared with experimental data. The in Theoretical study of structural, electronics and optical properties for these compounds allowed to understand the chemical changes that occurred in the ligand in the complexation process with the M2+ ion.