Filter-vial dispersive solid-phase extraction as a simplified clean-up for determination of ethylphenols in red wines

In-vial filtration with dispersive solid-phase extraction (d-SPE) clean-up of QuEChERS (quick, easy, cheap, effective, rugged and safe) extracts is proposed for the determination of ethylphenols (EPs) in red wines. Analytes were extracted from 5 mL wine sample (previously alkalinized with 0.5% sodiu...

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Detalles Bibliográficos
Autores: Fontana, Ariel Ramón, Bottini, Ambrosio Rubén
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2017
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/40008
Acceso en línea:http://hdl.handle.net/11336/40008
Access Level:acceso abierto
Palabra clave:Brett Character
D-Spe with In-Vial Filtration
Ethylphenols
Liquid Chromatography
Quechers
Wine
https://purl.org/becyt/ford/2.11
https://purl.org/becyt/ford/2
Descripción
Sumario:In-vial filtration with dispersive solid-phase extraction (d-SPE) clean-up of QuEChERS (quick, easy, cheap, effective, rugged and safe) extracts is proposed for the determination of ethylphenols (EPs) in red wines. Analytes were extracted from 5 mL wine sample (previously alkalinized with 0.5% sodium hydroxide) using 5 mL acetonitrile. For phase separation, 1.5 g NaCl and 4 g anhydrous MgSO4 were added. Then, a 0.5 mL aliquot of the partitioned supernatant was cleaned-up using d-SPE and in-vial filtration with a combination of anhydrous CaCl2 (100 mg) and primary-secondary amine (PSA, 25 mg) as sorbents. The proposed method provided limits of quantification (LOQs) ranging from 0.024 to 0.04 mg L−1. Considering matrix-matched calibration as quantification technique, the recoveries (accuracy) ranged between 73% and 116%. The method was applied for the determination of EPs in 15 commercial wines of Argentina, where 4-EP was quantified at concentrations ranging from 0.25 to 3.01 mg L−1.