Simultaneous quantification of 4-ethylphenol and ethanethiol in wines by headspace amperometric measurements

Simultaneous analysis of 4-ethylphenol and ethanethiol has been carried out since they often coexist in wine samples producing significant organoleptic defects. Dual working screen-printed electrodes have been used for this aim. An activated fullerene C60 modified screen-printed carbon electrode (AC...

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Detalles Bibliográficos
Autores: Portugal Gómez, Paula, Domínguez Renedo, Olga, Alonso Lomillo, Mª Asunción
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:España
Institución:Universidad de Burgos (UBU)
Repositorio:Repositorio Institucional de la Universidad de Burgos (RIUBU)
OAI Identifier:oai:riubu.ubu.es:10259/9287
Acceso en línea:http://hdl.handle.net/10259/9287
Access Level:acceso abierto
Palabra clave:4-Ethylphenol
Ethanethiol
Wine
Amperometry
Dual screen-printed carbon electrodes
Gas sensor
Chemistry, Analytic
Chemistry, Physical and theoretical
Química analítica
Química física
Descripción
Sumario:Simultaneous analysis of 4-ethylphenol and ethanethiol has been carried out since they often coexist in wine samples producing significant organoleptic defects. Dual working screen-printed electrodes have been used for this aim. An activated fullerene C60 modified screen-printed carbon electrode (AC60/SPCE1) was used for the determination of 4-ethylphenol, while a cobalt (II) phthalocyanine modified SPCE (CoPh/SPCE2) was employed for ethanethiol detection. Headspace amperometric measurements were performed applying different potentials to the electrode system, which were coated by a commercial polyamide membrane immersed in supporting electrolyte, for the simultaneous and selective detection of both species in a single run. The constructed sensing dual system presented an exceptional detection performance with a capacity of detection of 2.7 mg/L and 0.2 mg/L for 4-ethyphenol and ethanethiol, respectively. The developed method was successfully applied for the simultaneous detection of both compounds in wine samples where it demonstrated a high degree of trueness and suitable efficiency.