Cobalt hexacyanoferrate: Compound stoichiometry, infrared spectroelectrochemistry, and photoinduced electron transfer

The cobalt hexacyanoferrate system, MhCokA[FeB(CN)6]l , (where M is an alkali metal cation, and the subscripts h, k, and l are stoichiometric coefficients, and A and B are the formal oxidation states of the Co and Fe metal sites in the structure) was shown to contain a rich series of compounds that...

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Detalhes bibliográficos
Autores: Lezna, Reynaldo Oscar, Romagnoli, Roberto, De Tacconi, Norma R., Rajeshwar, Krishnan
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2002
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/152053
Acesso em linha:http://hdl.handle.net/11336/152053
Access Level:acceso abierto
Palavra-chave:https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descrição
Resumo:The cobalt hexacyanoferrate system, MhCokA[FeB(CN)6]l , (where M is an alkali metal cation, and the subscripts h, k, and l are stoichiometric coefficients, and A and B are the formal oxidation states of the Co and Fe metal sites in the structure) was shown to contain a rich series of compounds that are inter-linked through various redox processes (involving both electron and cation transfer) either in the dark or under the near-infrared (IR) activation. These processes were studied by a combined use of cyclic voltammetry, in situ IR spectroelectrochemistry (using both intensity or potential modulation), and ex sim X-ray photoelectron spectroscopy.