Solvatipn of excess electrons in supercritical ammonia

Solvation of excess electrons in supercritical ammonia along the T = 450 K isotherm was investigated. Equilibrium aspects of solvation were analyzed using combined path integral-molecular dynamics techniques. Observations showed transition from localized to quasifree states at approximately one four...

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Detalles Bibliográficos
Autores: Rodriguez, J., Skaf, M.S., Laria, D.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2003
País:Argentina
Institución:Universidad Nacional de Buenos Aires. Facultad de Ciencias Exactas y Naturales
Repositorio:Biblioteca Digital (UBA-FCEN)
Idioma:inglés
OAI Identifier:paperaa:paper_00219606_v119_n12_p6044_Rodriguez
Acceso en línea:http://hdl.handle.net/20.500.12110/paper_00219606_v119_n12_p6044_Rodriguez
Access Level:acceso abierto
Palabra clave:Electrons
Ground state
Molecular dynamics
Supercritical fluids
Solvation
Ammonia
Descripción
Sumario:Solvation of excess electrons in supercritical ammonia along the T = 450 K isotherm was investigated. Equilibrium aspects of solvation were analyzed using combined path integral-molecular dynamics techniques. Observations showed transition from localized to quasifree states at approximately one fourth of the triple point density.