Mechanism and Kinetics of the OH• Radical Reaction with Formaldehyde Bound to an Si(OH)4 Monomer

In this work, quantum chemical methods are used to studythe reaction of OH• radicals with formaldehyde bound to the Si(OH)4monomer, as a model for silica mineral aerosols. The potential energysurfaces for the formaldehyde interaction with the surface modelhave been carefully spanned, and minima and...

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Detalles Bibliográficos
Autores: Cristina Iuga, Rodolfo Esquivel Olea, Annik Vivier Bunge
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2008
País:México
Institución:Universidad Autónoma Metropolitana
Repositorio:Redalyc-UAM
OAI Identifier:oai:redalyc.org:47552106
Acceso en línea:https://www.redalyc.org/articulo.oa?id=47552106
Access Level:acceso abierto
Palabra clave:Química
OH radicals
formaldehyde
rate constants
Mineral aerosols
radical reactions
Descripción
Sumario:In this work, quantum chemical methods are used to studythe reaction of OH• radicals with formaldehyde bound to the Si(OH)4monomer, as a model for silica mineral aerosols. The potential energysurfaces for the formaldehyde interaction with the surface modelhave been carefully spanned, and minima and maxima were evaluated.Both the H-abstraction and OH-addition paths are shown to becomplex reactions, which involve the formation of a reactant complexin the entrance channel and a product complex in the exit channel. Inthe main reaction channel, formaldehyde binds to the silanol groupsand then reacts with OH free radicals to form a water molecule anda bound formyl radical. We show that the rate constant for the Habstractionreaction is an order of magnitude smaller when formaldehydeis bound to Si(OH)4 than in the gas phase, while the rate constantfor the addition reaction is still about five orders of magnitudesmaller. Thus, the branching ratio between abstraction and addition isnot significantly altered in the presence of the silicate surface model.