Upper critical fields in a FeSeO.5TeO.5 superconducting single crystal
A single crystal with a nominal composition FeSe0.5Te0.5 was obtained by the Bridgman method. A quartz ampulla with the sample inside was vacuum-sealed and maintained at 1050 !C for 37 h to homogenize the sample. Subsequently, the quartz ampulla with the sample was moved with a speed of 2.2 mm/h to...
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| Tipo de recurso: | artículo |
| Estado: | Versión enviada para evaluación y publicación |
| Fecha de publicación: | 2013 |
| País: | México |
| Institución: | Centro de Investigación en Materiales Avanzados |
| Repositorio: | Fuente de Objetos Científicos Open Access del CIMAV |
| Idioma: | inglés |
| OAI Identifier: | oai:cimav.repositorioinstitucional.mx:1004/1005 |
| Acceso en línea: | http://cimav.repositorioinstitucional.mx/jspui/handle/1004/1005 |
| Access Level: | acceso abierto |
| Palabra clave: | info:eu-repo/classification/Superconductors/Crystal info:eu-repo/classification/cti/1 info:eu-repo/classification/cti/22 info:eu-repo/classification/cti/2299 info:eu-repo/classification/cti/229999 |
| Sumario: | A single crystal with a nominal composition FeSe0.5Te0.5 was obtained by the Bridgman method. A quartz ampulla with the sample inside was vacuum-sealed and maintained at 1050 !C for 37 h to homogenize the sample. Subsequently, the quartz ampulla with the sample was moved with a speed of 2.2 mm/h to a furnace which was at 450 !C. X-ray diffraction confirmed the tetragonal structure of the grown single crystal with the cleavage plane corresponding to the ab plane. Resistance measurements were carried out with magnetic fields from 0 to 9 T, applied parallel to the c axis and ab plane, respectively. A zero-field critical temperature Tc¼14K was determined. The upper critical field vs. temperature phase diagram was built for temperatures where the resistance drops to 90%, 50%, and 10% of the normal state resistance. The linear extrapolation to T¼0K gave upper critical fields of 57.2, 51.8, and 46.0 T for Hjjc axis and 109.6, 95.5, and 80.9 T for Hjjab. Applying the Werthamer–Helfand–Hohenberg (WHH) theory, upper critical fields of 39.6, 35.9, and 31.8 T and coherence lengths of 28.8, 30.3, and 32.1A ° were obtained for Hjjc; while for Hjjab, upper critical fields of 51.3, 40.7, and 37.5 T and coherence lengths of 22.3, 26.7, and 31.5A ° were obtained. The value of l0Hc2/kBTc calculated by the WHH theory exceeds the Pauli limit (1.84 T/K) indicating the unconventional nature of superconductivity. The activation energy U0 has two different rates of change with the applied magnetic field probably due to two different thermal activation mechanisms; the origin of which requires further investigation. A similar behavior is observed in the irreversibility lines. |
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