Synthesis of New Chiral Monosulfonamides Prepared from (11R,12R)- 11,12-Diamino-9,10-dihydro-9,10-ethanoanthracene and their Use as Ligands for Asymmetric Catalysis

New chiral monosulfonamides 6-16 containing (11R,12R)- diamino-9,10-dihydro-9,10-ethanoanthracene as carbon skeleton were prepared. Compounds 6-12, 15 and 16 were used as optically active ligands in the enantioselective ethylation of benzaldehyde. Moreover, the monosulfonamides 6-10 were tested in t...

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Detalles Bibliográficos
Autores: Gabriela Huelgas, Haydee Rojas Cabrera, Domingo Madrigal, Ratnasamy Somanathan, Pilar Guzmán, Aurelio Ortiz, Cecilia Anaya de Parrodi
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2013
País:México
Institución:Universidad de las Américas Puebla
Repositorio:Redalyc-UDLAP
OAI Identifier:oai:redalyc.org:47527412011
Acceso en línea:https://www.redalyc.org/articulo.oa?id=47527412011
Access Level:acceso abierto
Palabra clave:Química
Monosulfonamide
asymmetric catalysis
enantioselective addition
Descripción
Sumario:New chiral monosulfonamides 6-16 containing (11R,12R)- diamino-9,10-dihydro-9,10-ethanoanthracene as carbon skeleton were prepared. Compounds 6-12, 15 and 16 were used as optically active ligands in the enantioselective ethylation of benzaldehyde. Moreover, the monosulfonamides 6-10 were tested in the asymmetric transfer hydrogenation (ATH) of acetophenone with Rh(Cp*)L* complex.