A Mild and Efficient Method for the Chemoselective Synthesis of Acylals from Aromatic Aldehydes and their Deprotections Catalyzed by Sulfated Zirconia

Aldehydes can be converted to acylals by treatment with acetic anhydride in the presence ofsulfated zirconia in excellent yield at 0 oC. Ketones and aliphatic aldehydes are found to be unaffectedunder the reaction conditions. The deprotection of the resulting acylals is achieved using the samecataly...

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Detalles Bibliográficos
Autores: Guillermo E. Negrón, Laura N. Palacios, Deyanira Angeles, Rubén Gaviño, Leticia Lomas
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2005
País:México
Institución:Universidad Nacional Autónoma de México
Repositorio:Redalyc-UNAM
OAI Identifier:oai:redalyc.org:47549225
Acceso en línea:https://www.redalyc.org/articulo.oa?id=47549225
Access Level:acceso abierto
Palabra clave:Química
acylals
protection
deprotection
sulfated zirconia
Descripción
Sumario:Aldehydes can be converted to acylals by treatment with acetic anhydride in the presence ofsulfated zirconia in excellent yield at 0 oC. Ketones and aliphatic aldehydes are found to be unaffectedunder the reaction conditions. The deprotection of the resulting acylals is achieved using the samecatalyst at 60 oC. The catalyst can be reused in two cycles without losing its activity.