Water-soluble aryl-extended calix[4]pyrroles with unperturbed aromatic cavities: synthesis and binding studies

<p> We report the synthesis of a novel, water-soluble aryl-extended calix[4]pyrrole receptor. The water-solubilising groups are placed at the lower rim of the receptor, leaving the binding pocket unperturbed and open for modification. Binding studies were performed with a series of pyridine N-...

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Detalhes bibliográficos
Autores: Hernandez-Alonso, Daniel, Zankowski, Stanislaw, Adriaenssens, Louis, Ballester, Pau
Formato: artículo
Fecha de publicación:2014
País:España
Recursos:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/305854
Acesso em linha:http://hdl.handle.net/2072/305854
https://doi.org/10.1039/C4ob02108h
Access Level:acceso abierto
Palavra-chave:pyridine n-oxides
molecular recognition
anion
receptors
lectins
calixpyrroles
capsules
solvent
Descrição
Resumo:<p> We report the synthesis of a novel, water-soluble aryl-extended calix[4]pyrrole receptor. The water-solubilising groups are placed at the lower rim of the receptor, leaving the binding pocket unperturbed and open for modification. Binding studies were performed with a series of pyridine N-oxides. These studies revealed the ability of the receptor to bind neutral and charged N-oxides in basified water with stability constants higher than 10(4) M-1.</p>