Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen

The creation of complex hollow nanostructures with precise control over size and shape represents a great challenge in supramolecular soft materials. Here, we have further developed a bioinspired methodology for the formation of aqueous nanotubes of well-defined dimensions and pore coating through t...

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Detalhes bibliográficos
Autores: Aparicio, Fátima, Sancho-Casado, Irene, Chamorro, Paula B., González-Sánchez, Marina, Pujals, Silvia, Vega-Mayoral, Victor, González-Rodríguez, David
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/368921
Acesso em linha:http://hdl.handle.net/10261/368921
https://api.elsevier.com/content/abstract/scopus_id/85204532029
Access Level:acceso abierto
Palavra-chave:Supramolecular
Amphiphiles
Encapsulation
Nanotubes
Self-assembly
http://metadata.un.org/sdg/3
Ensure healthy lives and promote well-being for all at all ages
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spelling Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic LumenAparicio, FátimaSancho-Casado, IreneChamorro, Paula B.González-Sánchez, MarinaPujals, SilviaVega-Mayoral, VictorGonzález-Rodríguez, DavidSupramolecularAmphiphilesEncapsulationNanotubesNanotubesSelf-assemblyhttp://metadata.un.org/sdg/3Ensure healthy lives and promote well-being for all at all agesThe creation of complex hollow nanostructures with precise control over size and shape represents a great challenge in supramolecular soft materials. Here, we have further developed a bioinspired methodology for the formation of aqueous nanotubes of well-defined dimensions and pore coating through the self-assembly of amphiphiles that are chemically programmed with complementary nucleobases. These nanotubes are endowed with a hydrophobic lumen, whose diameter can be expanded as a function of the monomer length, in which apolar dyes can be efficiently encapsulated.This work was supported by MCIN (PID2020-116921GB-I00, TED2021-132602B-I00) and AEI (PID2020-116112RJ-I00). F.A. is grateful to MCIN and Next Generation EU funding for a “Ramon-y-Cajal” fellowship (RyC-2021-031538-I). P. B. C. is grateful to the Comunidad de Madrid for the PEJ-2017-AI/IND-6246 contract. V V.-M. acknowledges grants TED2021-131906A-100, PID2021-128313OB-I00 and CNS2022-136191, funded by the Spanish Ministry of Science, Innovation and Universities (10.13039/501100011033), as well as support from the Regional Government of Madrid (2019-T2/IND-12737).Peer reviewedJohn Wiley & Sons0000-0002-4237-30110000-0002-3119-41570000-0002-2292-07940000-0001-8626-0775Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202420242024info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Publisher's versioninfo:eu-repo/semantics/publishedVersionhttp://hdl.handle.net/10261/368921https://api.elsevier.com/content/abstract/scopus_id/85204532029reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)InglésChemistry (Weinheim an der Bergstrasse, Germany)https://doi.org/10.1002/chem.202402365Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/3689212026-05-22T06:33:51Z
dc.title.none.fl_str_mv Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
title Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
spellingShingle Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
Aparicio, Fátima
Supramolecular
Amphiphiles
Encapsulation
Nanotubes
Nanotubes
Self-assembly
http://metadata.un.org/sdg/3
Ensure healthy lives and promote well-being for all at all ages
title_short Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
title_full Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
title_fullStr Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
title_full_unstemmed Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
title_sort Self-Assembly of Chemically Programmed Amphiphiles into Aqueous Nanotubes with a Lipophilic Lumen
dc.creator.none.fl_str_mv Aparicio, Fátima
Sancho-Casado, Irene
Chamorro, Paula B.
González-Sánchez, Marina
Pujals, Silvia
Vega-Mayoral, Victor
González-Rodríguez, David
author Aparicio, Fátima
author_facet Aparicio, Fátima
Sancho-Casado, Irene
Chamorro, Paula B.
González-Sánchez, Marina
Pujals, Silvia
Vega-Mayoral, Victor
González-Rodríguez, David
author_role author
author2 Sancho-Casado, Irene
Chamorro, Paula B.
González-Sánchez, Marina
Pujals, Silvia
Vega-Mayoral, Victor
González-Rodríguez, David
author2_role author
author
author
author
author
author
dc.contributor.none.fl_str_mv 0000-0002-4237-3011
0000-0002-3119-4157
0000-0002-2292-0794
0000-0001-8626-0775
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv Supramolecular
Amphiphiles
Encapsulation
Nanotubes
Nanotubes
Self-assembly
http://metadata.un.org/sdg/3
Ensure healthy lives and promote well-being for all at all ages
topic Supramolecular
Amphiphiles
Encapsulation
Nanotubes
Nanotubes
Self-assembly
http://metadata.un.org/sdg/3
Ensure healthy lives and promote well-being for all at all ages
description The creation of complex hollow nanostructures with precise control over size and shape represents a great challenge in supramolecular soft materials. Here, we have further developed a bioinspired methodology for the formation of aqueous nanotubes of well-defined dimensions and pore coating through the self-assembly of amphiphiles that are chemically programmed with complementary nucleobases. These nanotubes are endowed with a hydrophobic lumen, whose diameter can be expanded as a function of the monomer length, in which apolar dyes can be efficiently encapsulated.
publishDate 2024
dc.date.none.fl_str_mv 2024
2024
2024
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Publisher's version
info:eu-repo/semantics/publishedVersion
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/368921
https://api.elsevier.com/content/abstract/scopus_id/85204532029
url http://hdl.handle.net/10261/368921
https://api.elsevier.com/content/abstract/scopus_id/85204532029
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv Chemistry (Weinheim an der Bergstrasse, Germany)
https://doi.org/10.1002/chem.202402365
Sí
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.publisher.none.fl_str_mv John Wiley & Sons
publisher.none.fl_str_mv John Wiley & Sons
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
_version_ 1869424915099156480
score 15.81155

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