In situ study on enhanced plastic deformability of Lanthanum-doped Bismuth ferrite processed by flash sintering

BiFeO3 is a promising multiferroic material for versatile device applications due to its co-existence of magnetic (i.e., antiferromagnetic) and ferroelectric ordering at room temperature. While its functional properties have been extensively investigated, the exploration of its mechanical behavior w...

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Detalles Bibliográficos
Autores: Yang, Bo, Sánchez-Jiménez, Pedro E., Niu, Tongjun, Sun, Tianyi, Shang, Zhongxia, Cho, Jaehun, Perejón, Antonio, Shen, Chao, Pérez-Maqueda, Luis A., Tsakalakos, Thomas, Wang, Haiyan, Zhang, Xinghang
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2024
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/376124
Acceso en línea:http://hdl.handle.net/10261/376124
https://api.elsevier.com/content/abstract/scopus_id/85182696558
Access Level:acceso embargado
Palabra clave:Perovskite
Bismuth ferrite
Deformation mechanism
Flash sintering
In-situ compression test
Descripción
Sumario:BiFeO3 is a promising multiferroic material for versatile device applications due to its co-existence of magnetic (i.e., antiferromagnetic) and ferroelectric ordering at room temperature. While its functional properties have been extensively investigated, the exploration of its mechanical behavior was limited mostly to the thin-film form of BiFeO3. In this work, we conducted in situ micropillar compression experiments to investigate the deformation behavior of La-doped BiFeO3 (La-BFO) samples processed by both conventional and flash sintering methods. The conventionally sintered La-BFO exhibited limited deformability at room temperature and 450 °C. In contrast, the deformability of the flash-sintered La-BFO specimens was substantially improved by nearly 100% at both testing temperatures. Detailed post-mortem studies suggest that preexisting dislocations and wide anti-phase boundaries introduced during flash sintering can toughen flash-sintered La-BFO by easing dislocation migration and ferroelastic domain switching. This study provides a fresh perspective to design an advanced multifunctional system with improved mechanical properties.