The organic chemistry of poly(1H-pyrazol-1-yl)methanes

Since their first synthesis by Hückel (1937) and the first systematic exploration by Trofimenko (1970), interest in poly(1H-pyrazol-1-yl)methanes (bis, tris and tetrakis) has increased dramatically. This review focuses on the synthesis and reactivity of these ligands and contains 541 different struc...

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Detalhes bibliográficos
Autores: Díez Barra, Enrique, Claramunt, Rosa M., Elguero, José, López, Concepción, Alkorta, Ibón, Hoz Ayuso, Antonio de la
Formato: artículo
Fecha de publicación:2017
País:España
Recursos:Universidad de Castilla-La Mancha
Repositorio:RUIdeRA. Repositorio Institucional de la UCLM
OAI Identifier:oai:ruidera.uclm.es:10578/12911
Acesso em linha:https://hdl.handle.net/10578/12911
Access Level:acceso abierto
Palavra-chave:Pyrazoles
Pyrazolylmethanes
Bis(1H-pyrazol-1-yl)methanes
Tris(1H-pyrazol-1-yl)methanes
Tetrakis(1H-pyrazol-1-yl)methanes
Metal ligands
X-ray structures
Descrição
Resumo:Since their first synthesis by Hückel (1937) and the first systematic exploration by Trofimenko (1970), interest in poly(1H-pyrazol-1-yl)methanes (bis, tris and tetrakis) has increased dramatically. This review focuses on the synthesis and reactivity of these ligands and contains 541 different structures and 271 references. After a brief historical introduction, the synthesis, reactivity, and nature of the coordinated metals are described along with some properties of these compounds, particularly the complete set of X-ray molecular structures. All of the formulae are represented to show the extraordinary richness of poly(1H-pyrazol-1-yl)methanes and to promote the use of the already known poly(1H-pyrazol-1-yl)methanes in coordination chemistry and the design of new ligands with the reported procedures.