Catalytic Photoinduced Intramolecular Decarboxylative and Desulfonylative sp3Allylation Enabled by Sulfinate Salts

Herein, we describe a catalytic intramolecular decarboxylative/desulfonylative sp3 allylation triggered by sulfinate salts under light irradiation. The reaction is likely enabled by a non-classical, radical-polar crossover reaction, allowing to rapidly and reliably access valuable allyl architecture...

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Detalhes bibliográficos
Autores: Haut, Franz-Lucas, Mega, Riccardo S, Estornell, Joan V, Martin, Ruben
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2023
País:España
Recursos:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/534683
Acesso em linha:http://hdl.handle.net/2072/534683
https://doi.org/10.1002/anie.202304084
Access Level:acceso abierto
Palavra-chave:Química
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Descrição
Resumo:Herein, we describe a catalytic intramolecular decarboxylative/desulfonylative sp3 allylation triggered by sulfinate salts under light irradiation. The reaction is likely enabled by a non-classical, radical-polar crossover reaction, allowing to rapidly and reliably access valuable allyl architectures from readily accessible precursors. The protocol is characterized by its operational simplicity and scalability, employing abundant, commercially available catalysts