Polymer/surfactant assisted self-assembly of nanoparticles into Langmuir–Blodgett films

[EN]We studied the ability of poly(octadecene-co-maleic anhydride) (PMAO) and a Gemini surfactant [C18H37 (CH3)2NþBr e(CH2)2eNþBr (CH3)2 C18H37] (18-2-18) to assist in the self-assembly process of CdSe quantum dots (QDs) at the airewater interface. Results show that, while QD agglomeration is genera...

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Detalles Bibliográficos
Autores: Alejo Cuesta, María Teresa, Merchán Moreno, María Dolores, Velázquez Salicio, María Mercedes, Pérez Hernández, J.A
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2013
País:España
Institución:Universidad de Salamanca (USAL)
Repositorio:GREDOS. Repositorio Institucional de la Universidad de Salamanca
OAI Identifier:oai:gredos.usal.es:10366/158025
Acceso en línea:http://hdl.handle.net/10366/158025
Access Level:acceso abierto
Palabra clave:Polymers
Nanostructures
Thin film
Atomic force microscopy (AFM)
Electron microscopy (SEM)
Descripción
Sumario:[EN]We studied the ability of poly(octadecene-co-maleic anhydride) (PMAO) and a Gemini surfactant [C18H37 (CH3)2NþBr e(CH2)2eNþBr (CH3)2 C18H37] (18-2-18) to assist in the self-assembly process of CdSe quantum dots (QDs) at the airewater interface. Results show that, while QD agglomeration is generally inhibited by the addition of these components to the Langmuir monolayer of QDs, structure of the film transferred onto mica by the LangmuireBlodgett method is strongly affected by the dewetting process. Nucleation-and-growth of holes and spinodal-like dewetting were respectively observed in the presence of either PMAO or 18-2-18. When PMAO/18-2-18 mixtures were used, both mechanisms were allowed; nevertheless, even in films prepared with mixtures of low polymer contents, characteristic morphology from the polymer dewetting route prevailed.