Multiwavelength light-responsive Au/B-TiO2 Janus micromotors

Conventional photocatalytic micromotors are limited to the use of specific wavelengths of light due to their narrow light absorption spectrum, which limits their effectiveness for applications in biomedicine and environmental remediation. We present a multiwavelength light-responsive Janus micromoto...

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Detalles Bibliográficos
Autores: Jang, Bumjin, Hong, Ayoung, KangHa, Eun Kang, Alcantara, Carlos, Charreyron, Samuel, Mushtaq, Fajer, Pellicer, Eva|||0000-0002-8901-0998, Büchel, Robert, Sort, Jordi|||0000-0003-1213-3639, Lee, Sung Sik, Nelson, Bradley J.|||0000-0001-9070-6987, Pané i Vidal, Salvador|||0000-0003-0147-8287
Tipo de recurso: artículo
Fecha de publicación:2017
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:203510
Acceso en línea:https://ddd.uab.cat/record/203510
https://dx.doi.org/urn:doi:10.1021/acsnano.7b02177
Access Level:acceso abierto
Palabra clave:Au/B-TiO2 Janus micromotors
Black TiO2
Micromotors
Multiwavelengths
Photocatalysis
Descripción
Sumario:Conventional photocatalytic micromotors are limited to the use of specific wavelengths of light due to their narrow light absorption spectrum, which limits their effectiveness for applications in biomedicine and environmental remediation. We present a multiwavelength light-responsive Janus micromotor consisting of a black TiO₂ microsphere asymmetrically coated with a thin Au layer. The black TiO₂ microspheres exhibit absorption ranges between 300 and 800 nm. The Janus micromotors are propelled by light, both in H₂O₂ solutions and in pure H₂O over a broad range of wavelengths including UV, blue, cyan, green, and red light. An analysis of the particles' motion shows that the motor speed decreases with increasing wavelength, which has not been previously realized. A significant increase in motor speed is observed when exploiting the entire visible light spectrum (.