Pseudophosphorylation of single residues of the J-domain of regulates the holding/folding balance of the Hsc70 system

The Hsp70 system is essential for maintaining protein homeostasis and comprises a central Hsp70 and two accessory proteins that belong to the J-domain protein (JDP) and nucleotide exchange factor families. Posttranslational modifications offer a means to tune the activity of the system. We explore h...

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Detalhes bibliográficos
Autores: Velasco-Carneros, Lorea|||0000-0002-1296-9498, Bernardo-Seisdedos, Ganeko, Maréchal, Jean-Didier|||0000-0002-8344-9043, Millet, Oscar, Moro, Fernando, Muga, Arturo|||0000-0003-0345-6882
Formato: artículo
Fecha de publicación:2024
País:España
Recursos:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:312430
Acesso em linha:https://ddd.uab.cat/record/312430
https://dx.doi.org/urn:doi:10.1002/pro.5105
Access Level:acceso abierto
Palavra-chave:Chaperone
DNAJA2
Hsc70
J-domain
Phosphorylation
Protein folding
Descrição
Resumo:The Hsp70 system is essential for maintaining protein homeostasis and comprises a central Hsp70 and two accessory proteins that belong to the J-domain protein (JDP) and nucleotide exchange factor families. Posttranslational modifications offer a means to tune the activity of the system. We explore how phosphorylation of specific residues of the J-domain of DNAJA2, a class A JDP, regulates Hsc70 activity using biochemical and structural approaches. Among these residues, we find that pseudophosphorylation of Y10 and S51 enhances the holding/folding balance of the Hsp70 system, reducing cochaperone collaboration with Hsc70 while maintaining the holding capacity. Truly phosphorylated J domains corroborate phosphomimetic variant effects. Notably, distinct mechanisms underlie functional impacts of these DNAJA2 variants. Pseudophosphorylation of Y10 induces partial disordering of the J domain, whereas the S51E substitution weakens essential DNAJA2-Hsc70 interactions without a large structural reorganization of the protein. S51 phosphorylation might be class-specific, as all cytosolic class A human JDPs harbor a phosphorylatable residue at this position.