Recombination dynamics in ZnO nanowires: Surfaces states versus mode quality factor

In this work, we investigate the influence of finite size on the recombinations dynamics of ZnO nanowires. We demonstrate that diameter as well as lenght of nanowires determine the lifetime of the neutral donor bound excitons. Our findings suggest that while the length is mainly responsible for diff...

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Bibliographic Details
Authors: Reparaz, J. S., Güell Vilà, Frank, Wagner, M. R., Callsen, G., Kirste, R., Claramunt Ruiz, Sergi, Morante i Lleonart, Joan Ramon, Hoffmann, A.
Format: article
Status:Published version
Publication Date:2010
Country:España
Institution:Universidad de Barcelona
Repository:Dipòsit Digital de la UB
OAI Identifier:oai:diposit.ub.edu:2445/33836
Online Access:https://hdl.handle.net/2445/33836
Access Level:Open access
Keyword:Òxid de zinc
Nanotecnologia
Nanoestructures
Ciència dels materials
Zinc oxide
Nanotechnology
Nanostructures
Materials science
Description
Summary:In this work, we investigate the influence of finite size on the recombinations dynamics of ZnO nanowires. We demonstrate that diameter as well as lenght of nanowires determine the lifetime of the neutral donor bound excitons. Our findings suggest that while the length is mainly responsible for different mode quality factors of the cavity-like nanowires, the diameter determines the influence of surface states as alternative recombinations channels for the optical modes trapped in the nanocavity. In addition, comparing nanowires grown using different catalyst we show that the surfaces states strongly depend on each precursor characteristics.