Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit

6 figures, 1 table.-- © 2020. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/

Detalles Bibliográficos
Autores: Samprón, Iván, Diego Poza, Luis F. de, García Labiano, Francisco, Izquierdo Pantoja, María Teresa, Abad Secades, Alberto, Adánez Elorza, Juan
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2020
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/217738
Acceso en línea:http://hdl.handle.net/10261/217738
Access Level:acceso abierto
Palabra clave:Biomass
Chemical-looping gasification
Syngas
Tar
Biofuels
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spelling Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unitSamprón, IvánDiego Poza, Luis F. deGarcía Labiano, FranciscoIzquierdo Pantoja, María TeresaAbad Secades, AlbertoAdánez Elorza, JuanBiomassChemical-looping gasificationSyngasTarBiofuels6 figures, 1 table.-- © 2020. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/Biomass Chemical Looping Gasification is a novel technology allowing high quality syngas production at autothermal conditions without CO2 emissions to the atmosphere and low tar generation. This work compiles gasification results corresponding to 38 h of continuous operation in a 1.5 kWth unit using pine wood as fuel and a synthetic Fe-based oxygen carrier, Fe20Al. The main operating conditions such as temperature (T = 820–940 °C), steam-to-biomass ratio (S/B = 0.05–0.65), and oxygen-to-biomass ratio (λ = 0.2–0.6) were analyzed at steady state conditions using a novel method for controlling oxygen in the process. A syngas composed by 37% H2, 21% CO, 34% CO2 and 7% CH4, and tars below 2 g/Nm3 could be obtained at autothermal conditions, leading to a syngas yield of 0.8 Nm3/kg dry biomass and a cold gas efficiency of 68%. The material maintained a high reactivity although some Fe lost was observed.This work was supported by ENE2017-89473-R AEI/FEDER, UE. I. Samprón thanks the Spanish Ministerio de Ciencia, Innovación y Universidades (MICIU) for the PRE-086217 pre-doctoral fellowship.Peer reviewedElsevierMinisterio de Ciencia, Innovación y Universidades (España)European CommissionAgencia Estatal de Investigación (España)Diego Poza, Luis F. de [0000-0002-4106-3441]García Labiano, Francisco [0000-0002-5857-0976]Izquierdo Pantoja, María Teresa [0000-0002-2408-2528]Abad Secades, Alberto [0000-0002-4995-3473]Adánez Elorza, Juan [0000-0002-6287-098X]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202020202020info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Postprintinfo:eu-repo/semantics/acceptedVersionhttp://hdl.handle.net/10261/217738reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Inglés#PLACEHOLDER_PARENT_METADATA_VALUE#info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/ENE2017-89473-Rhttp://dx.doi.org/10.1016/j.biortech.2020.123908Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/2177382026-05-22T06:33:51Z
dc.title.none.fl_str_mv Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
title Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
spellingShingle Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
Samprón, Iván
Biomass
Chemical-looping gasification
Syngas
Tar
Biofuels
title_short Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
title_full Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
title_fullStr Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
title_full_unstemmed Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
title_sort Biomass Chemical Looping Gasification of pine wood using a synthetic Fe2O3/Al2O3 oxygen carrier in a continuous unit
dc.creator.none.fl_str_mv Samprón, Iván
Diego Poza, Luis F. de
García Labiano, Francisco
Izquierdo Pantoja, María Teresa
Abad Secades, Alberto
Adánez Elorza, Juan
author Samprón, Iván
author_facet Samprón, Iván
Diego Poza, Luis F. de
García Labiano, Francisco
Izquierdo Pantoja, María Teresa
Abad Secades, Alberto
Adánez Elorza, Juan
author_role author
author2 Diego Poza, Luis F. de
García Labiano, Francisco
Izquierdo Pantoja, María Teresa
Abad Secades, Alberto
Adánez Elorza, Juan
author2_role author
author
author
author
author
dc.contributor.none.fl_str_mv Ministerio de Ciencia, Innovación y Universidades (España)
European Commission
Agencia Estatal de Investigación (España)
Diego Poza, Luis F. de [0000-0002-4106-3441]
García Labiano, Francisco [0000-0002-5857-0976]
Izquierdo Pantoja, María Teresa [0000-0002-2408-2528]
Abad Secades, Alberto [0000-0002-4995-3473]
Adánez Elorza, Juan [0000-0002-6287-098X]
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv Biomass
Chemical-looping gasification
Syngas
Tar
Biofuels
topic Biomass
Chemical-looping gasification
Syngas
Tar
Biofuels
description 6 figures, 1 table.-- © 2020. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/
publishDate 2020
dc.date.none.fl_str_mv 2020
2020
2020
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Postprint
info:eu-repo/semantics/acceptedVersion
format article
status_str acceptedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/217738
url http://hdl.handle.net/10261/217738
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv #PLACEHOLDER_PARENT_METADATA_VALUE#
info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/ENE2017-89473-R
http://dx.doi.org/10.1016/j.biortech.2020.123908
Sí
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.publisher.none.fl_str_mv Elsevier
publisher.none.fl_str_mv Elsevier
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,81155

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