Carbon dioxide capture from combustion flue gases with a calcium oxide chemical loop. Experimental results and process development

Post-combustion carbonate looping processes are based on the capture of carbon dioxide from the flue gases of an existing power plant in a circulating fluidized bed reactor (CFB) of calcium oxide (the carbonator) particles. The calcination of calcium carbonate in a new oxy-fired CFBC power plant reg...

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Detalhes bibliográficos
Autores: Alonso Carreño, Mónica, Rodríguez Gómez, Nuria, González García, Belén, Grasa Adiego, Gemma, Murillo Villuendas, Ramón, Abanades García, Juan Carlos
Formato: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2010
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/221291
Acesso em linha:http://hdl.handle.net/10261/221291
Access Level:acceso abierto
Palavra-chave:CO2 capture
Carbonate looping
Carbonation
Calcination
Pilot testing
Descrição
Resumo:Post-combustion carbonate looping processes are based on the capture of carbon dioxide from the flue gases of an existing power plant in a circulating fluidized bed reactor (CFB) of calcium oxide (the carbonator) particles. The calcination of calcium carbonate in a new oxy-fired CFBC power plant regenerates the sorbent (calcium oxide particles) and obtains high purity carbon dioxide. This communication presents experimental results from a small test facility (30 kWt) operated in continuous mode using two interconnected CFB reactors as carbonator and calciner. Capture efficiencies between 70 and 97% have been obtained under realistic flue gas conditions in the carbonator reactor (temperatures around 650 °C). The similarity between process conditions and those existing in CFBC power plants should allow a rapid scaling up of this technology. The next steps for this process development are also outlined. © 2009 Elsevier Ltd. All rights reserved.