Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications

López Sánchez, Jesús; Del Campo Garcia, Angel Adolfo; Quesada, Adrián; Rivelles, Alejandro; Abuín, Manuel; Sainz, Raquel; Sebastiani-Tofano, Eugenia; Rubio Zuazo, Juan; Ochoa Guerrero, Diego A.|||0000-0002-8756-9704; Fernández Lozano, José Francisco; García García, José Eduardo|||0000-0002-1232-1739; Rubio Marcos, Fernando

Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications

The concept of multiphysics, where materials respond to diverse external stimuli, such as magnetic fields, electric fields, light irradiation, stress, heat, and chemical reactions, plays a fundamental role in the development of innovative devices. Nanomanufacturing, especially in low-dimensional sys...

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Autores:	López Sánchez, Jesús, Del Campo Garcia, Angel Adolfo, Quesada, Adrián, Rivelles, Alejandro, Abuín, Manuel, Sainz, Raquel, Sebastiani-Tofano, Eugenia, Rubio Zuazo, Juan, Ochoa Guerrero, Diego A.\|\|\|0000-0002-8756-9704, Fernández Lozano, José Francisco, García García, José Eduardo\|\|\|0000-0002-1232-1739, Rubio Marcos, Fernando
Tipo de recurso:	artículo
Fecha de publicación:	2024
País:	España
Institución:	Universitat Politècnica de Catalunya (UPC)
Repositorio:	UPCommons. Portal del coneixement obert de la UPC
Idioma:	inglés
OAI Identifier:	oai:upcommons.upc.edu:2117/406806
Acceso en línea:	https://hdl.handle.net/2117/406806 https://dx.doi.org/10.1021/acsami.4c02551
Access Level:	acceso abierto
Palabra clave:	Ferromagnetic materials Multiferroics Epitaxial thin films Magneto-structural coupling Photostrictive materials Charge distribution modulation Ferroelectric domain wall commutation Materials ferromagnètics Àrees temàtiques de la UPC::Enginyeria dels materials::Materials funcionals

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spelling	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applicationsLópez Sánchez, JesúsDel Campo Garcia, Angel AdolfoQuesada, AdriánRivelles, AlejandroAbuín, ManuelSainz, RaquelSebastiani-Tofano, EugeniaRubio Zuazo, JuanOchoa Guerrero, Diego A.\|\|\|0000-0002-8756-9704Fernández Lozano, José FranciscoGarcía García, José Eduardo\|\|\|0000-0002-1232-1739Rubio Marcos, FernandoFerromagnetic materialsMultiferroicsEpitaxial thin filmsMagneto-structural couplingPhotostrictive materialsCharge distribution modulationFerroelectric domain wall commutationMaterials ferromagnèticsÀrees temàtiques de la UPC::Enginyeria dels materials::Materials funcionalsThe concept of multiphysics, where materials respond to diverse external stimuli, such as magnetic fields, electric fields, light irradiation, stress, heat, and chemical reactions, plays a fundamental role in the development of innovative devices. Nanomanufacturing, especially in low-dimensional systems, enhances the synergistic interactions taking place on the nanoscale. Light–matter interaction, rather than electric fields, holds great promise for achieving low-power, wireless control over magnetism, solving two major technological problems: the feasibility of electrical contacts at smaller scales and the undesired heating of the devices. Here, we shed light on the remarkable reversible modulation of magnetism using visible light in epitaxial Fe3O4/BaTiO3 heterostructure. This achievement is underpinned by the convergence of two distinct mechanisms. First, the magnetoelastic effect, triggered by ferroelectric domain switching, induces a proportional change in coercivity and remanence upon laser illumination. Second, light–matter interaction induces charged ferroelectric domain walls’ electrostatic decompensations, acting intimately on the magnetization of the epitaxial Fe3O4 film by magnetoelectric coupling. Crucially, our experimental results vividly illustrate the capability to manipulate magnetic properties using visible light. This concomitant mechanism provides a promising avenue for low-intensity visible-light manipulation of magnetism, offering potential applications in multiferroic devices.20242024-04-1720242024-04-19journal articlehttp://purl.org/coar/resource_type/c_6501VoRhttp://purl.org/coar/version/c_970fb48d4fbd8a85info:eu-repo/semantics/articleapplication/pdfapplication/pdfhttps://hdl.handle.net/2117/406806https://dx.doi.org/10.1021/acsami.4c02551reponame:UPCommons. Portal del coneixement obert de la UPCinstname:Universitat Politècnica de Catalunya (UPC)Inglésengopen accesshttp://purl.org/coar/access_right/c_abf2Attribution 4.0 Internationalhttp://creativecommons.org/licenses/by/4.0/info:eu-repo/semantics/openAccessoai:upcommons.upc.edu:2117/4068062026-05-27T15:37:01Z
dc.title.none.fl_str_mv	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications
title	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications
spellingShingle	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications López Sánchez, Jesús Ferromagnetic materials Multiferroics Epitaxial thin films Magneto-structural coupling Photostrictive materials Charge distribution modulation Ferroelectric domain wall commutation Materials ferromagnètics Àrees temàtiques de la UPC::Enginyeria dels materials::Materials funcionals
title_short	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications
title_full	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications
title_fullStr	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications
title_full_unstemmed	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications
title_sort	Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications
dc.creator.none.fl_str_mv	López Sánchez, Jesús Del Campo Garcia, Angel Adolfo Quesada, Adrián Rivelles, Alejandro Abuín, Manuel Sainz, Raquel Sebastiani-Tofano, Eugenia Rubio Zuazo, Juan Ochoa Guerrero, Diego A.\|\|\|0000-0002-8756-9704 Fernández Lozano, José Francisco García García, José Eduardo\|\|\|0000-0002-1232-1739 Rubio Marcos, Fernando
author	López Sánchez, Jesús
author_facet	López Sánchez, Jesús Del Campo Garcia, Angel Adolfo Quesada, Adrián Rivelles, Alejandro Abuín, Manuel Sainz, Raquel Sebastiani-Tofano, Eugenia Rubio Zuazo, Juan Ochoa Guerrero, Diego A.\|\|\|0000-0002-8756-9704 Fernández Lozano, José Francisco García García, José Eduardo\|\|\|0000-0002-1232-1739 Rubio Marcos, Fernando
author_role	author
author2	Del Campo Garcia, Angel Adolfo Quesada, Adrián Rivelles, Alejandro Abuín, Manuel Sainz, Raquel Sebastiani-Tofano, Eugenia Rubio Zuazo, Juan Ochoa Guerrero, Diego A.\|\|\|0000-0002-8756-9704 Fernández Lozano, José Francisco García García, José Eduardo\|\|\|0000-0002-1232-1739 Rubio Marcos, Fernando
author2_role	author author author author author author author author author author author
dc.subject.none.fl_str_mv	Ferromagnetic materials Multiferroics Epitaxial thin films Magneto-structural coupling Photostrictive materials Charge distribution modulation Ferroelectric domain wall commutation Materials ferromagnètics Àrees temàtiques de la UPC::Enginyeria dels materials::Materials funcionals
topic	Ferromagnetic materials Multiferroics Epitaxial thin films Magneto-structural coupling Photostrictive materials Charge distribution modulation Ferroelectric domain wall commutation Materials ferromagnètics Àrees temàtiques de la UPC::Enginyeria dels materials::Materials funcionals
description	The concept of multiphysics, where materials respond to diverse external stimuli, such as magnetic fields, electric fields, light irradiation, stress, heat, and chemical reactions, plays a fundamental role in the development of innovative devices. Nanomanufacturing, especially in low-dimensional systems, enhances the synergistic interactions taking place on the nanoscale. Light–matter interaction, rather than electric fields, holds great promise for achieving low-power, wireless control over magnetism, solving two major technological problems: the feasibility of electrical contacts at smaller scales and the undesired heating of the devices. Here, we shed light on the remarkable reversible modulation of magnetism using visible light in epitaxial Fe3O4/BaTiO3 heterostructure. This achievement is underpinned by the convergence of two distinct mechanisms. First, the magnetoelastic effect, triggered by ferroelectric domain switching, induces a proportional change in coercivity and remanence upon laser illumination. Second, light–matter interaction induces charged ferroelectric domain walls’ electrostatic decompensations, acting intimately on the magnetization of the epitaxial Fe3O4 film by magnetoelectric coupling. Crucially, our experimental results vividly illustrate the capability to manipulate magnetic properties using visible light. This concomitant mechanism provides a promising avenue for low-intensity visible-light manipulation of magnetism, offering potential applications in multiferroic devices.
publishDate	2024
dc.date.none.fl_str_mv	2024 2024-04-17 2024 2024-04-19
dc.type.none.fl_str_mv	journal article http://purl.org/coar/resource_type/c_6501 VoR http://purl.org/coar/version/c_970fb48d4fbd8a85
dc.type.openaire.fl_str_mv	info:eu-repo/semantics/article
format	article
dc.identifier.none.fl_str_mv	https://hdl.handle.net/2117/406806 https://dx.doi.org/10.1021/acsami.4c02551
url	https://hdl.handle.net/2117/406806 https://dx.doi.org/10.1021/acsami.4c02551
dc.language.none.fl_str_mv	Inglés eng
language_invalid_str_mv	Inglés
language	eng
dc.rights.none.fl_str_mv	open access http://purl.org/coar/access_right/c_abf2 Attribution 4.0 International http://creativecommons.org/licenses/by/4.0/
dc.rights.openaire.fl_str_mv	info:eu-repo/semantics/openAccess
rights_invalid_str_mv	open access http://purl.org/coar/access_right/c_abf2 Attribution 4.0 International http://creativecommons.org/licenses/by/4.0/
eu_rights_str_mv	openAccess
dc.format.none.fl_str_mv	application/pdf application/pdf
dc.source.none.fl_str_mv	reponame:UPCommons. Portal del coneixement obert de la UPC instname:Universitat Politècnica de Catalunya (UPC)
instname_str	Universitat Politècnica de Catalunya (UPC)
reponame_str	UPCommons. Portal del coneixement obert de la UPC
collection	UPCommons. Portal del coneixement obert de la UPC
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score	15,301603

Concomitant light-reversible magnetic response in multiferroic oxide heterostructures for multiphysics applications

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