Extraction of antimony from a hydrochloric acid side stream of copper electro-refining by hydrolysis

This work explores the feasibility of recovering antimony, present in a side stream of hydrochloric acid resulting from a copper electro-refining process, by hydrolysis with water. A range of variables that can affect the process have been studied. According to the results, under optimal conditions...

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Detalles Bibliográficos
Autores: Díaz, Eduardo, Maldonado Calvo, José A., Gallardo Fuentes, José María, Paúl Escolano, Antonio
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2023
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/146033
Acceso en línea:https://hdl.handle.net/11441/146033
https://doi.org/10.1016/j.hydromet.2023.106076
Access Level:acceso abierto
Palabra clave:Antimony metallurgy
Antimony oxychloride
Hydrolysis
Copper electro-refining
Descripción
Sumario:This work explores the feasibility of recovering antimony, present in a side stream of hydrochloric acid resulting from a copper electro-refining process, by hydrolysis with water. A range of variables that can affect the process have been studied. According to the results, under optimal conditions (pH = 0.645 T = 34 °C), antimony extraction yield is 94.4%. The reaction product is amorphous, with antimony content close to 70% and Cl and O contents similar to the stoichiometric ratios of complex oxychloride compounds. Moreover, significant amounts of arsenic and bismuth have been revealed. The presence of bismuth affects the extraction performance, while arsenic impairs its potential commercialisation.