Applicability of the closed-circuit accumulation chamber technique to measure radon surface exhalation rate under laboratory conditions

A layer of phosphogypsum was placed at the bottom of two large volume boxes. This system allowed to measure the surface radon exhalation from phosphogypsum without altering the emitting material. The limits and optimal setup of the closed-circuit accumulation chamber technique were thoroughly studie...

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Detalles Bibliográficos
Autores: Gutiérrez Álvarez, Isidoro, Martín Domínguez, José Enrique, Adame, José Antonio, Grossi, Claudia|||0000-0001-6678-4440, Vargas Drechsler, Arturo|||0000-0002-2576-9671, Bolívar Raya, Juan Pedro
Tipo de recurso: artículo
Fecha de publicación:2020
País:España
Institución:Universitat Politècnica de Catalunya (UPC)
Repositorio:UPCommons. Portal del coneixement obert de la UPC
Idioma:inglés
OAI Identifier:oai:upcommons.upc.edu:2117/329484
Acceso en línea:https://hdl.handle.net/2117/329484
https://dx.doi.org/10.1016/j.radmeas.2020.106284
Access Level:acceso abierto
Palabra clave:Radon
Chemical laboratories
Radon exhalation
Phosphogypsum
Linearity time
Radó
Laboratoris químics
Àrees temàtiques de la UPC::Enginyeria química
Àrees temàtiques de la UPC::Enginyeria química::Química física
Descripción
Sumario:A layer of phosphogypsum was placed at the bottom of two large volume boxes. This system allowed to measure the surface radon exhalation from phosphogypsum without altering the emitting material. The limits and optimal setup of the closed-circuit accumulation chamber technique were thoroughly studied. More precisely, the performance of different radon exhalation fitting methods was analyzed in the reference exhalation boxes, employing different measurement devices and three smaller operational accumulation chambers. As expected, the best approach to obtain the radon exhalation rate depends upon the effective decay constant of the measurement system and the time employed to perform the measurement. The time until the linear approximation can no longer be applied was scrutinized. Although this approximation is usually applied routinely in the literature, the effective time constant of the chamber is often not low enough for the linear fit to be applied safely, providing statistically acceptable measurements that can lead to significative underestimations of the radon exhalation rate.