Solvent-Controlled Switching of Cycloisomerization to Transposition in the Ag/Cu-Promoted Reaction of Terminal α-Allenols

We report herein a study on the Ag/Cu-catalyzed reactivity of α-allenols. The focus was the development of new methodologies for cyclization and/or transposition of this moiety. By simple solvent switch, the divergent preparation of dihydrofurans and 3-halo-3-alkenals in a controlled manner has been...

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Detalhes bibliográficos
Autores: Toledano Pinedo, Mireia, Anatóliev, Hristo, Martínez Del Campo, Teresa, Almendros, Pedro
Formato: artículo
Fecha de publicación:2019
País:España
Recursos:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/8288
Acesso em linha:https://hdl.handle.net/20.500.14352/8288
Access Level:acceso abierto
Palavra-chave:allene
dihydrofurans and 3-halo-3-alkenals
Química orgánica (Química)
2306 Química Orgánica
Descrição
Resumo:We report herein a study on the Ag/Cu-catalyzed reactivity of α-allenols. The focus was the development of new methodologies for cyclization and/or transposition of this moiety. By simple solvent switch, the divergent preparation of dihydrofurans and 3-halo-3-alkenals in a controlled manner has been reached.