Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal)
24 páginas.- 8 figuras.- 4 tablas.- 122 referencias.- Electronic supplementary material The online version of this article (https://doi.org/10.1007/s11356-020-09235-9) contains supplementary material, which is available to authorized users.
| Autores: | , , , , |
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| Tipo de recurso: | artículo |
| Estado: | Versión aceptada para publicación |
| Fecha de publicación: | 2020 |
| País: | España |
| Institución: | Consejo Superior de Investigaciones Científicas (CSIC) |
| Repositorio: | DIGITAL.CSIC. Repositorio Institucional del CSIC |
| OAI Identifier: | oai:digital.csic.es:10261/212390 |
| Acceso en línea: | http://hdl.handle.net/10261/212390 |
| Access Level: | acceso abierto |
| Palabra clave: | Aliphatic hydrocarbons Coastal lagoons Hopanes Lignin Polycyclic aromatic hydrocarbons Steranes |
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Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal)Kumar, MukeshBoski, TomaszGonzález-Vila, Francisco JavierRosa Arranz, José M. de laGonzález-Pérez, José AntonioAliphatic hydrocarbonsCoastal lagoonsHopanesLigninPolycyclic aromatic hydrocarbonsSteranes24 páginas.- 8 figuras.- 4 tablas.- 122 referencias.- Electronic supplementary material The online version of this article (https://doi.org/10.1007/s11356-020-09235-9) contains supplementary material, which is available to authorized users.Sedimentary organic matter (OM) origin and molecular composition provide useful information to understand carbon cycling in coastal wetlands. Core sediments from threors’ Contributionse transects along Ria Formosa lagoon intertidal zone were analysed using analytical pyrolysis (Py-GC/MS) to determine composition, distribution and origin of sedimentary OM. The distribution of alkyl compounds (alkanes, alkanoic acids and alkan-2-ones), polycyclic aromatic hydrocarbons (PAHs), lignin-derived methoxyphenols, linear alkylbenzenes (LABs), steranes and hopanes indicated OM inputs to the intertidal environment from natural—autochthonous and allochthonous—as well as anthropogenic. Several n-alkane geochemical indices used to assess the distribution of main OM sources (terrestrial and marine) in the sediments indicate that algal and aquatic macrophyte derived OM inputs dominated over terrigenous plant sources. The lignin-derived methoxyphenol assemblage, dominated by vinylguaiacol and vinylsyringol derivatives in all sediments, points to large OM contribution from higher plants. The spatial distributions of PAHs (polyaromatic hydrocarbons) showed that most pollution sources were mixed sources including both pyrogenic and petrogenic. Low carbon preference indexes (CPI > 1) for n-alkanes, the presence of UCM (unresolved complex mixture) and the distribution of hopanes (C29–C36) and steranes (C27–C29) suggested localized petroleum-derived hydrocarbon inputs to the core sediments. Series of LABs were found in most sediment samples also pointing to domestic sewage anthropogenic contributions to the sediment OM. © 2020, Springer-Verlag GmbH Germany, part of Springer Nature.The authors received funding from EU Erasmus Mundus Joint Doctorate fellowship (FUECA, University of Cadiz, Spain) for Mukesh Kumar. The research was supported by EU contract numbers FP7-ENV-2011, Grant agreement no: 282845 and FP7- 534 ENV-2012 Grant agreement no: 308392 and also from MINECO project INTERCARBON (CGL2016-78937-R).Peer reviewedSpringer NatureEuropean CommissionUniversidad de CádizGonzález-Vila, Francisco Javier [0000-0002-6320-5391]Rosa Arranz, José M. de la [0000-0003-2857-2345]González-Pérez, José Antonio [0000-0001-7607-1444]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202020202020info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Postprintinfo:eu-repo/semantics/acceptedVersionhttp://hdl.handle.net/10261/212390reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Inglés#PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE##PLACEHOLDER_PARENT_METADATA_VALUE#info:eu-repo/grantAgreement/EC/FP7/282845info:eu-repo/grantAgreement/EC/FP7/308392info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/CGL2016-78937-Rhttp://dx.doi.org/10.1007/s11356-020-09235-9Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/2123902026-05-22T06:33:51Z |
| dc.title.none.fl_str_mv |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) |
| title |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) |
| spellingShingle |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) Kumar, Mukesh Aliphatic hydrocarbons Coastal lagoons Hopanes Lignin Polycyclic aromatic hydrocarbons Steranes |
| title_short |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) |
| title_full |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) |
| title_fullStr |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) |
| title_full_unstemmed |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) |
| title_sort |
Discerning natural and anthropogenic organic matter inputs to salt marsh sediments of Ria Formosa lagoon (South Portugal) |
| dc.creator.none.fl_str_mv |
Kumar, Mukesh Boski, Tomasz González-Vila, Francisco Javier Rosa Arranz, José M. de la González-Pérez, José Antonio |
| author |
Kumar, Mukesh |
| author_facet |
Kumar, Mukesh Boski, Tomasz González-Vila, Francisco Javier Rosa Arranz, José M. de la González-Pérez, José Antonio |
| author_role |
author |
| author2 |
Boski, Tomasz González-Vila, Francisco Javier Rosa Arranz, José M. de la González-Pérez, José Antonio |
| author2_role |
author author author author |
| dc.contributor.none.fl_str_mv |
European Commission Universidad de Cádiz González-Vila, Francisco Javier [0000-0002-6320-5391] Rosa Arranz, José M. de la [0000-0003-2857-2345] González-Pérez, José Antonio [0000-0001-7607-1444] Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72] |
| dc.subject.none.fl_str_mv |
Aliphatic hydrocarbons Coastal lagoons Hopanes Lignin Polycyclic aromatic hydrocarbons Steranes |
| topic |
Aliphatic hydrocarbons Coastal lagoons Hopanes Lignin Polycyclic aromatic hydrocarbons Steranes |
| description |
24 páginas.- 8 figuras.- 4 tablas.- 122 referencias.- Electronic supplementary material The online version of this article (https://doi.org/10.1007/s11356-020-09235-9) contains supplementary material, which is available to authorized users. |
| publishDate |
2020 |
| dc.date.none.fl_str_mv |
2020 2020 2020 |
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info:eu-repo/semantics/article http://purl.org/coar/resource_type/c_6501 Postprint info:eu-repo/semantics/acceptedVersion |
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article |
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acceptedVersion |
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http://hdl.handle.net/10261/212390 |
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http://hdl.handle.net/10261/212390 |
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Inglés |
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Inglés |
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#PLACEHOLDER_PARENT_METADATA_VALUE# #PLACEHOLDER_PARENT_METADATA_VALUE# #PLACEHOLDER_PARENT_METADATA_VALUE# info:eu-repo/grantAgreement/EC/FP7/282845 info:eu-repo/grantAgreement/EC/FP7/308392 info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/CGL2016-78937-R http://dx.doi.org/10.1007/s11356-020-09235-9 Sí |
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info:eu-repo/semantics/openAccess |
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openAccess |
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Springer Nature |
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Springer Nature |
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reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC instname:Consejo Superior de Investigaciones Científicas (CSIC) |
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Consejo Superior de Investigaciones Científicas (CSIC) |
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DIGITAL.CSIC. Repositorio Institucional del CSIC |
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DIGITAL.CSIC. Repositorio Institucional del CSIC |
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