1,8-Hydrogen Atom Transfer Promoted by N-Radicals in (1-4)-O-Disaccharide Models

The nitrogen-centered radical generated by reaction of an N-sulfonamidate, attached to C-6 of a hexopyranose in a disaccharide model, with (diacetoxyiodo)benzene (DIB) and iodine undergoes a novel regio- and stereoselective intramolecular 1,8-hydrogen atom transfer (HAT) reaction to promote the func...

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Detalles Bibliográficos
Autores: León, Elisa I., Martín, Ángeles, Pérez-Martín, Inés, Suárez, Ernesto
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2011
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/199610
Acceso en línea:http://hdl.handle.net/10261/199610
Access Level:acceso abierto
Palabra clave:Carbohydrates
Radical reactions
Hydrogen transfer
Radicals
Descripción
Sumario:The nitrogen-centered radical generated by reaction of an N-sulfonamidate, attached to C-6 of a hexopyranose in a disaccharide model, with (diacetoxyiodo)benzene (DIB) and iodine undergoes a novel regio- and stereoselective intramolecular 1,8-hydrogen atom transfer (HAT) reaction to promote the functionalization of remote positions.