Facile synthesis of heterogeneous indium nanoparticles for formate production via CO2 electroreduction

In this study, a simple and scalable method to obtain heterogeneous indium nanoparticles and carbon-supported indium nanoparticles under mild conditions is described. Physicochemical characterization by X-ray diffraction (XRD), X-ray photoelectron microscopy (XPS), scanning electron microscopy (SEM)...

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Detalles Bibliográficos
Autores: Pérez-Sequera, Ana Cristina, Díaz-Pérez, Manuel Antonio, Lara Angulo, Mayra Anabel, Holgado, Juan P., Serrano Ruiz, Juan Carlos
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universidad Loyola Andalucía
Repositorio:Brújula
OAI Identifier:oai:repositorio.uloyola.es:20.500.12412/4015
Acceso en línea:https://hdl.handle.net/20.500.12412/4015
Access Level:acceso abierto
Palabra clave:Indium catalysts
CO2 electroreduction
Carbon-supported materials
Heterogeneous catalysts
Formate production
CO2 conversion
Descripción
Sumario:In this study, a simple and scalable method to obtain heterogeneous indium nanoparticles and carbon-supported indium nanoparticles under mild conditions is described. Physicochemical characterization by X-ray diffraction (XRD), X-ray photoelectron microscopy (XPS), scanning electron microscopy (SEM) and transmission electron microscopy (TEM) revealed heterogeneous morphologies for the In nanoparticles in all cases. Apart from In0, XPS revealed the presence of oxidized In species on the carbon-supported samples, whereas these species were not observed for the unsupported samples. The best-in-class catalyst (In50/C50) exhibited a high formate Faradaic efficiency (FE) near the unit (above 97%) at