Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis

[EN] A multifunctional material design, integrating catalytic as well as auxiliary magnetic susception and contactless thermal sensing functionalities, unlocks catalyst-specific heating and thermometry for spatially proximate solid catalysts in a single reactor. The new concept alleviates temperatur...

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Autores: Garcia-Farpon, Marcos, Peláez-Fernández, Raquel, Atakan, Burak, Zaldo, Carlos, Recio-Ballesteros, Veronica, Prieto González, Gonzalo|||0000-0002-0956-3040
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/205208
Acceso en línea:https://riunet.upv.es/handle/10251/205208
Access Level:acceso abierto
Palabra clave:Catalyst-specific heating
Ethene
Materials
Reactor
Tandem catalysis
Thermometry
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spelling Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysisGarcia-Farpon, MarcosPeláez-Fernández, RaquelAtakan, BurakZaldo, CarlosRecio-Ballesteros, VeronicaPrieto González, Gonzalo|||0000-0002-0956-3040Catalyst-specific heatingEtheneMaterialsReactorTandem catalysisThermometry[EN] A multifunctional material design, integrating catalytic as well as auxiliary magnetic susception and contactless thermal sensing functionalities, unlocks catalyst-specific heating and thermometry for spatially proximate solid catalysts in a single reactor. The new concept alleviates temperature incompatibilities in tandem catalysis, as showcased for the direct production of propene from ethene, via sequential olefin dimerization and metathesis reactions.This research has received funding from the Spanish Ministry of Science and Innovation (projects ERC2018-092838 and PID2021-128090OB-C21) and the European Research Council (ERC) under the Horizon 2020 research and innovation programme (ERC-CoG-TANDEng; grant agreement 864195). M. G. F. acknowledges support by the Spanish Ministry of Education through predoctoral grant FPU17/04701. R. P. acknowledges support by the Conselleria Valenciana de Innovacion, Universidades, Ciencia y Sociedad Digital through postdoctoral fellowship CIAPOS/2021/92. P. Marin (Univ. Oviedo) and A. M. Luque (ITQ) are acknowledged for contributions to the development of the meshed geometry and model for CFD simulations, and C. Cascales (ICMM) for discussions on phosphor design. XAS experiments were performed at the CL AE SS beamline at ALBA Synchrotron (Barcelona, Spain) with the collaboration of ALBA staff. W. Henao, C. Marini and G. Agostini are acknowledged for guidance with data collection and XAS data reduction. E. Torregrosa (ITQ) is acknowledged for assistance with induction heating experiments.The Royal Society of ChemistryInstituto Universitario Mixto de Tecnología QuímicaEuropean CommissionEuropean Research CouncilAgencia Estatal de InvestigaciónUniversitat Politècnica de ValènciaMinisterio de Ciencia, Innovación y UniversidadesConselleria de Innovación, Universidades, Ciencia y Sociedad Digital, Generalitat ValencianaRepositorio Institucional de la Universitat Politècnica de València Riunet20232023-09-26journal articlehttp://purl.org/coar/resource_type/c_6501VoRhttp://purl.org/coar/version/c_970fb48d4fbd8a85info:eu-repo/semantics/articleapplication/pdfhttps://riunet.upv.es/handle/10251/205208reponame:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valénciainstname:Universitat Politècnica de València (UPV)InglésengAgencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023 PID2021-128090OB-C21 SOLUCIONES NO CONVENCIONALES EN TERMOMETRIA DE ALTA TEMPERATURA BASADA EN LUMINISCENCIA PARA APLICACIONES DE INTERES INDUSTRIALEuropean Commission https://doi.org/10.13039/501100000780 H2020 864195 Engineering catalyst interoperability in next-generation tandem reactions for intensified chemical processesMinisterio de Ciencia, Innovación y Universidades https://doi.org/10.13039/100014440 FPU17%2F04701Agencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 ERC2018-092838 Nuevos nanomateriales para la termometría remota y específica en procesos catalíticosGeneralitat Valenciana https://doi.org/10.13039/501100003359 Programa para la promoción de la investigación científica, el desarrollo tecnológico y la innovación en la Comunitat Valenciana CIAPOS%2F2021%2F92open accesshttp://purl.org/coar/access_right/c_abf2Reconocimiento (by)http://creativecommons.org/licenses/by/4.0/info:eu-repo/semantics/openAccessoai:riunet.upv.es:10251/2052082026-06-13T07:49:27Z
dc.title.none.fl_str_mv Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
title Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
spellingShingle Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
Garcia-Farpon, Marcos
Catalyst-specific heating
Ethene
Materials
Reactor
Tandem catalysis
Thermometry
title_short Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
title_full Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
title_fullStr Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
title_full_unstemmed Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
title_sort Multifunctional materials for catalyst-specific heating and thermometry in tandem catalysis
dc.creator.none.fl_str_mv Garcia-Farpon, Marcos
Peláez-Fernández, Raquel
Atakan, Burak
Zaldo, Carlos
Recio-Ballesteros, Veronica
Prieto González, Gonzalo|||0000-0002-0956-3040
author Garcia-Farpon, Marcos
author_facet Garcia-Farpon, Marcos
Peláez-Fernández, Raquel
Atakan, Burak
Zaldo, Carlos
Recio-Ballesteros, Veronica
Prieto González, Gonzalo|||0000-0002-0956-3040
author_role author
author2 Peláez-Fernández, Raquel
Atakan, Burak
Zaldo, Carlos
Recio-Ballesteros, Veronica
Prieto González, Gonzalo|||0000-0002-0956-3040
author2_role author
author
author
author
author
dc.contributor.none.fl_str_mv Instituto Universitario Mixto de Tecnología Química
European Commission
European Research Council
Agencia Estatal de Investigación
Universitat Politècnica de València
Ministerio de Ciencia, Innovación y Universidades
Conselleria de Innovación, Universidades, Ciencia y Sociedad Digital, Generalitat Valenciana
Repositorio Institucional de la Universitat Politècnica de València Riunet
dc.subject.none.fl_str_mv Catalyst-specific heating
Ethene
Materials
Reactor
Tandem catalysis
Thermometry
topic Catalyst-specific heating
Ethene
Materials
Reactor
Tandem catalysis
Thermometry
description [EN] A multifunctional material design, integrating catalytic as well as auxiliary magnetic susception and contactless thermal sensing functionalities, unlocks catalyst-specific heating and thermometry for spatially proximate solid catalysts in a single reactor. The new concept alleviates temperature incompatibilities in tandem catalysis, as showcased for the direct production of propene from ethene, via sequential olefin dimerization and metathesis reactions.
publishDate 2023
dc.date.none.fl_str_mv 2023
2023-09-26
dc.type.none.fl_str_mv journal article
http://purl.org/coar/resource_type/c_6501
VoR
http://purl.org/coar/version/c_970fb48d4fbd8a85
dc.type.openaire.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv https://riunet.upv.es/handle/10251/205208
url https://riunet.upv.es/handle/10251/205208
dc.language.none.fl_str_mv Inglés
eng
language_invalid_str_mv Inglés
language eng
dc.relation.none.fl_str_mv Agencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023 PID2021-128090OB-C21 SOLUCIONES NO CONVENCIONALES EN TERMOMETRIA DE ALTA TEMPERATURA BASADA EN LUMINISCENCIA PARA APLICACIONES DE INTERES INDUSTRIAL
European Commission https://doi.org/10.13039/501100000780 H2020 864195 Engineering catalyst interoperability in next-generation tandem reactions for intensified chemical processes
Ministerio de Ciencia, Innovación y Universidades https://doi.org/10.13039/100014440 FPU17%2F04701
Agencia Estatal de Investigación http://dx.doi.org/10.13039/501100011033 ERC2018-092838 Nuevos nanomateriales para la termometría remota y específica en procesos catalíticos
Generalitat Valenciana https://doi.org/10.13039/501100003359 Programa para la promoción de la investigación científica, el desarrollo tecnológico y la innovación en la Comunitat Valenciana CIAPOS%2F2021%2F92
dc.rights.none.fl_str_mv open access
http://purl.org/coar/access_right/c_abf2
Reconocimiento (by)
http://creativecommons.org/licenses/by/4.0/
dc.rights.openaire.fl_str_mv info:eu-repo/semantics/openAccess
rights_invalid_str_mv open access
http://purl.org/coar/access_right/c_abf2
Reconocimiento (by)
http://creativecommons.org/licenses/by/4.0/
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv The Royal Society of Chemistry
publisher.none.fl_str_mv The Royal Society of Chemistry
dc.source.none.fl_str_mv reponame:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
instname:Universitat Politècnica de València (UPV)
instname_str Universitat Politècnica de València (UPV)
reponame_str RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
collection RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
repository.name.fl_str_mv
repository.mail.fl_str_mv
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